Preparation of TiO2-CNT-Ag Ternary Composite Film with Enhanced Photocatalytic Activity via Plasma-Enhanced Chemical Vapor Deposition

被引：14
作者：
Lang, Jianghua [1 ]
Takahashi, Kazuma [1 ]
Kubo, Masaru [2 ]
Shimada, Manabu [2 ]
机构：
[1] Hiroshima Univ, Grad Sch Engn, Dept Chem Engn, 1-4-1 Kagamiyama, Higashihiroshima, Hiroshima 7398527, Japan
[2] Hiroshima Univ, Grad Sch Adv Sci & Engn, Chem Engn Program, 1-4-1 Kagamiyama, Higashihiroshima, Hiroshima 7398527, Japan
来源：
CATALYSTS | 2022年 / 12卷 / 05期
基金：
日本学术振兴会;
关键词：
thin film deposition; nanoparticles; aerosols; photocatalysis; SILVER NANOPARTICLES; CARBON NANOTUBE; TIO2; FILMS; ANATASE TIO2; THIN-FILMS; HETEROJUNCTION; PHOTODEGRADATION; DEGRADATION;
D O I：
10.3390/catal12050508
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
In this study, a TiO2-CNT-Ag ternary composite film was successfully synthesized using the plasma-enhanced chemical vapor deposition method by simultaneously feeding a carbon nanotube (CNT)/Ag suspension and titanium tetraisopropoxide gas. The prepared TiO2-CNT-Ag film was characterized by scanning electron microscopy, transmission electron microscopy, energy-dispersive X-ray spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction, and ultraviolet-visible spectroscopy. Moreover, the Ag/Ti ratio of the film was confirmed using an inductivity-coupled plasma optical emission spectrometer. The performance of the TiO2-composite film for the degradation of rhodamine 6G under simulated solar light irradiation was evaluated. The rate constant of the prepared TiO2-CNT-Ag for rhodamine 6G degradation was approximately 1.8 times greater than that of prepared TiO2. This result indicates that the addition of CNT and Ag significantly improved the photocatalytic activity of the prepared films.
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页数：13
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