Zeolitic imidazolate frameworks derived nitrogen doped porous carbon for electrochemical reduction of CO2

被引:2
作者
Zhong, Xi [1 ]
Zhong, Heng [1 ]
Jin, Fangming [1 ,2 ,3 ]
机构
[1] Shanghai Jiao Tong Univ, Sch Environm Sci & Engn, State Key Lab Met Matrix Composites, 800 Dongchuan RD, Shanghai 200240, Peoples R China
[2] Shanghai Inst Pollut Control & Ecol Secur, Shanghai 200092, Peoples R China
[3] Jiaxing Univ, Coll Biol Chem Sci & Engn, 56 South Yuexiu Rd, Jiaxing 314001, Peoples R China
来源
2ND INTERNATIONAL CONFERENCE ON AIR POLLUTION AND ENVIRONMENTAL ENGINEERING | 2020年 / 450卷
关键词
ELECTROCATALYSTS; ELECTROREDUCTION; DIOXIDE;
D O I
10.1088/1755-1315/450/1/012114
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The development of high-performance electrochemical materials plays an important role in CO2 reduction efficiency and cost effectiveness. In this work, nitrogen doped porous carbon matrix was designed and fabricated from zeolitic imidazolate frameworks (ZIF-8). Pyrolysis temperature was investigated to achieve the best performance to convert CO2 into CO. The suitable temperature is 700 degrees C which could make the catalyst containing good conductivity and activity. The highest Faradaic efficiency of CO is close to 25% at potential of -1.0 V.
引用
收藏
页数:5
相关论文
共 17 条
[1]   Exclusive Formation of Formic Acid from CO2 Electroreduction by a Tunable Pd-Sn Alloy [J].
Bai, Xiaofang ;
Chen, Wei ;
Zhao, Chengcheng ;
Li, Shenggang ;
Song, Yanfang ;
Ge, Ruipeng ;
Wei, Wei ;
Sun, Yuhan .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2017, 56 (40) :12219-12223
[2]   MOF derived carbon based nanocomposite materials as efficient electrocatalysts for oxygen reduction and oxygen and hydrogen evolution reactions [J].
Bhattacharyya, Sohini ;
Das, Chayanika ;
Maji, Tapas Kumar .
RSC ADVANCES, 2018, 8 (47) :26728-26754
[3]   Metal-Free Carbon Materials for CO2 Electrochemical Reduction [J].
Duan, Xiaochuan ;
Xu, Jiantie ;
Wei, Zengxi ;
Ma, Jianmin ;
Guo, Shaojun ;
Wang, Shuangyin ;
Liu, Huakun ;
Dou, Shixue .
ADVANCED MATERIALS, 2017, 29 (41)
[4]   Enhancing CO2 Electroreduction with the Metal-Oxide Interface [J].
Gao, Dunfeng ;
Zhang, Yi ;
Zhou, Zhiwen ;
Cai, Fan ;
Zhao, Xinfei ;
Huang, Wugen ;
Li, Yangsheng ;
Zhu, Junfa ;
Liu, Ping ;
Yang, Fan ;
Wang, Guoxiong ;
Bao, Xinhe .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2017, 139 (16) :5652-5655
[5]  
Hawxhurst C J, 2019, ANGEW CHEM
[6]  
Jeon H S, 2016, APPL CATAL B
[7]   Ag-Sn Bimetallic Catalyst with a Core-Shell Structure for CO2 Reduction [J].
Luc, Wesley ;
Collins, Charles ;
Wang, Siwen ;
Xin, Hongliang ;
He, Kai ;
Kang, Yijin ;
Jiao, Feng .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2017, 139 (05) :1885-1893
[8]   A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels [J].
Qiao, Jinli ;
Liu, Yuyu ;
Hong, Feng ;
Zhang, Jiujun .
CHEMICAL SOCIETY REVIEWS, 2014, 43 (02) :631-675
[9]   Mechanistic Insights into the Electrochemical Reduction of CO2 to CO on Nanostructured Ag Surfaces [J].
Rosen, Jonathan ;
Hutchings, Gregory S. ;
Lu, Qi ;
Rivera, Sean ;
Zhou, Yang ;
Vlachos, Dionisios G. ;
Jiao, Feng .
ACS CATALYSIS, 2015, 5 (07) :4293-4299
[10]   Ultrahigh Mass Activity for Carbon Dioxide Reduction Enabled by Gold-Iron Core-Shell Nanoparticles [J].
Sun, Kun ;
Cheng, Tao ;
Wu, Lina ;
Hu, Yongfeng ;
Zhou, Jigang ;
Maclennan, Aimee ;
Jiang, Zhaohua ;
Gao, Yunzhi ;
Goddard, William A., III ;
Wang, Zhijiang .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2017, 139 (44) :15608-15611