Plasmonic Nanocavity Organic Light-Emitting Diode with Significantly Enhanced Light Extraction, Contrast, Viewing Angle, Brightness, and Low-Glare

被引:54
作者
Ding, Wei [1 ]
Wang, Yuxuan [1 ]
Chen, Hao [1 ]
Chou, Stephen Y. [1 ]
机构
[1] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA
关键词
EXTERNAL-QUANTUM-EFFICIENCY; PHOTONIC CRYSTALS; SPONTANEOUS EMISSION; ANGULAR-DEPENDENCE; DEVICES; DISPLAYS; POLYMER; LITHOGRAPHY; CATHODE; LAYER;
D O I
10.1002/adfm.201400964
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
One central challenge in LEDs is to increase light extraction; but for display applications, other factors may have equal significance, such as ambient-light absorption, contrast, viewing angle, image sharpness, brightness, and low-glare. However, current LED structures enhance only some of the factors, while degrading the others. Here, a new organic LED (OLED) structure is proposed and demonstrated, with a novel plasmonic nanocavity, termed "plasmonic cavity with subwavelength hole-array" (PlaCSH), and exhibits experimentally signifi cant enhancements of all above factors with unprecedented performances. Compared to the conventional OLEDs (the same but without PlaCSH), PlaCSH-OLEDs achieve experimentally: i) 1.57-fold higher external-quantum-efficiency and light-extraction-efficiency (29%/32% without lens, 55%/60% with lens)-among the highest reported; ii) ambient-light absorption not only 2.5-fold higher but also broad-band (400 nm) and nearly angle and polarization independent, leading to lower-glare; iii) fivefold higher contrast (12 000 for 140 lux ambient-light); iv) viewing angle tunable by the cavity length; v) 1.86-fold higher normal-view-brightness; and vi) uniform color over all emission angles. The PlaCSH is an excellent optical antenna-excellent in both radiation and absorption of light. Furthermore, PlaCSH-OLEDs, a simple structure to produce, are fabricated using nanoimprint over large-area (approximate to 1000 cm(2)), hence scalable to wallpaper size.
引用
收藏
页码:6329 / 6339
页数:11
相关论文
共 58 条
[41]   HIGHLY EFFICIENT LIGHT-EMITTING-DIODES WITH MICROCAVITIES [J].
SCHUBERT, EF ;
HUNT, NEJ ;
MICOVIC, M ;
MALIK, RJ ;
SIVCO, DL ;
CHO, AY ;
ZYDZIK, GJ .
SCIENCE, 1994, 265 (5174) :943-945
[42]  
Schuller JA, 2010, NAT MATER, V9, P193, DOI [10.1038/NMAT2630, 10.1038/nmat2630]
[43]   Enhanced light out-coupling of organic light-emitting devices using embedded low-index grids [J].
Sun, Yiru ;
Forrest, Stephen R. .
NATURE PHOTONICS, 2008, 2 (08) :483-487
[44]   Roller nanoimprint lithography [J].
Tan, H ;
Gilbertson, A ;
Chou, SY .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B, 1998, 16 (06) :3926-3928
[45]  
Tsutsui T, 2001, ADV MATER, V13, P1149, DOI 10.1002/1521-4095(200108)13:15<1149::AID-ADMA1149>3.0.CO
[46]  
2-2
[47]   Surface plasmon enhanced light-emitting diode [J].
Vuckovic, J ;
Loncar, M ;
Scherer, A .
IEEE JOURNAL OF QUANTUM ELECTRONICS, 2000, 36 (10) :1131-1144
[48]   Unlocking the full potential of organic light-emitting diodes on flexible plastic [J].
Wang, Z. B. ;
Helander, M. G. ;
Qiu, J. ;
Puzzo, D. P. ;
Greiner, M. T. ;
Hudson, Z. M. ;
Wang, S. ;
Liu, Z. W. ;
Lu, Z. H. .
NATURE PHOTONICS, 2011, 5 (12) :753-757
[49]   High-power AlGaInN flip-chip light-emitting diodes [J].
Wierer, JJ ;
Steigerwald, DA ;
Krames, MR ;
O'Shea, JJ ;
Ludowise, MJ ;
Christenson, G ;
Shen, YC ;
Lowery, C ;
Martin, PS ;
Subramanya, S ;
Götz, W ;
Gardner, NF ;
Kern, RS ;
Stockman, SA .
APPLIED PHYSICS LETTERS, 2001, 78 (22) :3379-3381
[50]   III-nitride photonic-crystal light-emitting diodes with high extraction efficiency [J].
Wierer, Jonathan J., Jr. ;
David, Aurelien ;
Megens, Mischa M. .
NATURE PHOTONICS, 2009, 3 (03) :163-169