Effects of graphene oxide aggregates on hydration degree, sorptivity, and tensile splitting strength of cement paste
被引:178
作者:
Li, Xiangyu
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Taiyuan Univ Technol, Coll Architecture & Civil Engn, Taiyuan, Shanxi, Peoples R ChinaTaiyuan Univ Technol, Coll Architecture & Civil Engn, Taiyuan, Shanxi, Peoples R China
Li, Xiangyu
[1
]
Lu, Zeyu
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Hong Kong Univ Sci & Technol, Dept Civil & Environm Engn, Hong Kong, Hong Kong, Peoples R ChinaTaiyuan Univ Technol, Coll Architecture & Civil Engn, Taiyuan, Shanxi, Peoples R China
机构:
Hong Kong Univ Sci & Technol, Dept Civil & Environm Engn, Hong Kong, Hong Kong, Peoples R ChinaTaiyuan Univ Technol, Coll Architecture & Civil Engn, Taiyuan, Shanxi, Peoples R China
Li, Zongjin
[2
]
机构:
[1] Taiyuan Univ Technol, Coll Architecture & Civil Engn, Taiyuan, Shanxi, Peoples R China
[2] Hong Kong Univ Sci & Technol, Dept Civil & Environm Engn, Hong Kong, Hong Kong, Peoples R China
[3] Monash Univ, Dept Civil Engn, Clayton, Vic 3800, Australia
It has recently been found the graphene oxide (GO) aggregates form in cement paste due to the chemical cross-linking of calcium cations. Therefore, the effects of GO addition on the properties of cement based materials should be dependent on the properties of GO aggregates rather than GO nanosheets. In this study, GO aggregates were first characterized by particle size measurement. Then, the effects of GO aggregates on the degree of hydration, sorptivity, and tensile strength of cement paste were investigated. The aspect ratio of GO aggregates is much larger than that of the original GO nanosheets. Compared to plain cement paste, the increase of non-evaporable water content of the cement paste was found to be very limited, around 1.17% and 3.90% for cement pastes containing 0.02% and 0.04% by weight GO, respectively. The sorptivity of cement paste, especially the secondary sorptivity, was notably reduced for GO incorporated cement paste. The tensile strength was significantly improved by GO aggregates. Incorporation of 0.04% by weight GO increased the tensile strength by 67% compared to that of plain cement paste. (C) 2017 Elsevier Ltd. All rights reserved.
机构:
US EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
Chowdhury, Indranil
;
Duch, Matthew C.
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Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
Northwestern Univ, Dept Chem, Evanston, IL 60208 USA
Northwestern Univ, Dept Med, Evanston, IL 60208 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
Duch, Matthew C.
;
Mansukhani, Nikhita D.
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Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
Northwestern Univ, Dept Chem, Evanston, IL 60208 USA
Northwestern Univ, Dept Med, Evanston, IL 60208 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
Mansukhani, Nikhita D.
;
Hersam, Mark C.
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Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
Northwestern Univ, Dept Chem, Evanston, IL 60208 USA
Northwestern Univ, Dept Med, Evanston, IL 60208 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
Hersam, Mark C.
;
Bouchard, Dermont
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US EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
机构:
Middle E Tech Univ, Dept Civil Engn, TR-06531 Ankara, TurkeyNatl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USA
Erdogan, S. T.
;
Nie, X.
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机构:
Johns Hopkins Univ, Dept Phys, Baltimore, MD USANatl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USA
Nie, X.
;
Stutzman, P. E.
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Natl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USANatl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USA
Stutzman, P. E.
;
Garboczi, E. J.
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Natl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USANatl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USA
机构:
US EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
Chowdhury, Indranil
;
Duch, Matthew C.
论文数: 0引用数: 0
h-index: 0
机构:
Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
Northwestern Univ, Dept Chem, Evanston, IL 60208 USA
Northwestern Univ, Dept Med, Evanston, IL 60208 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
Duch, Matthew C.
;
Mansukhani, Nikhita D.
论文数: 0引用数: 0
h-index: 0
机构:
Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
Northwestern Univ, Dept Chem, Evanston, IL 60208 USA
Northwestern Univ, Dept Med, Evanston, IL 60208 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
Mansukhani, Nikhita D.
;
Hersam, Mark C.
论文数: 0引用数: 0
h-index: 0
机构:
Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
Northwestern Univ, Dept Chem, Evanston, IL 60208 USA
Northwestern Univ, Dept Med, Evanston, IL 60208 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
Hersam, Mark C.
;
Bouchard, Dermont
论文数: 0引用数: 0
h-index: 0
机构:
US EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USAUS EPA, Ecosyst Res Div, Natl Exposure Res Lab, Athens, GA 30605 USA
机构:
Middle E Tech Univ, Dept Civil Engn, TR-06531 Ankara, TurkeyNatl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USA
Erdogan, S. T.
;
Nie, X.
论文数: 0引用数: 0
h-index: 0
机构:
Johns Hopkins Univ, Dept Phys, Baltimore, MD USANatl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USA
Nie, X.
;
Stutzman, P. E.
论文数: 0引用数: 0
h-index: 0
机构:
Natl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USANatl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USA
Stutzman, P. E.
;
Garboczi, E. J.
论文数: 0引用数: 0
h-index: 0
机构:
Natl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USANatl Inst Stand & Technol, Inorgan Mat Grp, Mat & Construct Res Div, Bldg & Fire Res Lab, Gaithersburg, MD 20899 USA