Synthesis and photocatalytic property of a new 1D metal-organic polymer

被引：4
|
作者：
Yuan, Chun-Mei [1 ]
Yan, Meng-Ting [1 ]
Yuan, Fei [1 ]
Ling, Xin-Yu [2 ]
Zhou, Chun-Sheng [1 ]
Wang, Jun [2 ]
Cao, Bao-Yue [1 ]
Singh, Ayushi [3 ]
Kumar, Abhinav [3 ]
机构：
[1] Shangluo Univ, Shaanxi Key Lab Comprehens Utilizat Tailings Reso, Coll Chem Engn & Modern Mat, Shangluo 726000, Peoples R China
[2] Sichuan Univ Sci & Engn, Sch Chem & Environm Engn, Zigong, Peoples R China
[3] Univ Lucknow, Dept Chem, Fac Sci, Lucknow 226007, Uttar Pradesh, India
来源：
INORGANIC CHEMISTRY COMMUNICATIONS | 2019年 / 108卷
基金：
中国国家自然科学基金;
关键词：
Flexible carboxylate; Dye; Photocatalysis; DOS; COORDINATION POLYMERS; CRYSTAL-STRUCTURES; DEGRADATION; FRAMEWORK; ION; FLUORESCENCE; PERFORMANCE; ADSORPTION; REMOVAL; CD(II);
D O I：
10.1016/j.inoche.2019.107543
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
A new coordination polymer having composition [Zn(L)(phen)](n) (1) has been synthesized solvothermally usingl,4-bis(3-carboxylbenzyl)piperazine acid (H2L) and 1,10-phenanthroline (phen) and Zn(II) salt. The single-crystal X-ray diffraction studies revealed that 1 shows a 1D chain constructed by linking [Zn(phen)](2+) units via L ligands, which further generates a 2D layer through strong pi center dot center dot center dot pi stacking interactions operating between the pyridyl rings of phen ligands and piperazine ring from adjacent networks along the c axis. The photocatalytic property of 1 in photo-degradation of methyl violet (MV) has been explored. The possible mechanism has been addressed using density of states (DOS) and partial DOS (pDOS) calculations.
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页数：5
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