Large theoretical thermoelectric power factor of suspended single-layer MoS2

被引:82
作者
Babaei, Hasan [1 ,2 ]
Khodadadi, J. M. [2 ]
Sinha, Sanjiv [1 ]
机构
[1] Univ Illinois, Mech Sci & Engn Dept, Urbana, IL 61801 USA
[2] Auburn Univ, Dept Mech Engn, Auburn, AL 36849 USA
基金
美国国家科学基金会;
关键词
TRANSPORT;
D O I
10.1063/1.4901342
中图分类号
O59 [应用物理学];
学科分类号
摘要
We have calculated the semi-classical thermoelectric power factor of suspended single-layer (SL)-MoS2 utilizing electron relaxation times derived from ab initio calculations. Measurements of the thermoelectric power factor of SL-MoS2 on substrates reveal poor power factors. In contrast, we find the thermoelectric power factor of suspended SL-MoS2 to peak at similar to 2.8 x 10(4) mu W/m K-2 at 300K, at an electron concentration of 10(12) cm(-2). This figure is higher than that in bulk Bi2Te3, for example. Given its relatively high thermal conductivity, suspended SL-MoS2 may hold promise for in-plane thin-film Peltier coolers, provided reasonable mobilities can be realized. (C) 2014 AIP Publishing LLC.
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页数:5
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