Identification of failed cells inside PEMFC stacks in two cases: Anode/cathode crossover and anode/cooling compartment leak

被引:37
作者
Tian, Guangyu [2 ,3 ]
Wasterlain, Sebastien [1 ,4 ]
Candusso, Denis [1 ]
Harel, Fabien [1 ]
Hissel, Daniel [1 ,4 ]
Francois, Xavier [1 ,5 ]
机构
[1] FC LAB, F-90010 Belfort, France
[2] Tsinghua Univ, State Key Lab Automot Safety, Beijing 100084, Peoples R China
[3] Tsinghua Univ, Energy Dept Automot Engn, Beijing 100084, Peoples R China
[4] Univ Franche Comte, ENISYS Dept, FEMTO ST, CNRS,UMR 6174, F-25030 Besancon, France
[5] Univ Technol Belfort Montbeliard, Belfort, France
关键词
PEM fuel cell; Reliability; Diagnosis; Leakage; ELECTROLYTE FUEL-CELLS; DEGRADATION; DIAGNOSIS;
D O I
10.1016/j.ijhydene.2009.05.015
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Various PEMFC operating conditions can lead to irreversible damages as membrane break and gasket deterioration. If leak check procedures can highlight the lack of tightness in fuel cells, they are not appropriate to inform actually where the fault has occurred in the stacks. Thus, diagnosis procedures allowing the failed cells to be identified are needed. Then, these cells can be removed and replaced by safe ones. The article presents some descriptions of aged assemblies subjected to anode/cathode crossover and anode/cooling compartment leakage. Some experimental investigations are carried out with the goal to locate the defective cells. The open current voltages of the cells are monitored and analysed in different operating conditions. Experimental procedures combined with data analysis tools allow the detection of the failed cells, which show abnormal performance and voltage pattern when they are compared to the other safe cells. (C) 2009 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:2772 / 2776
页数:5
相关论文
共 10 条
[1]  
[Anonymous], MATLAB SOFTWARE
[2]   Novel evaluation method for degradation rate of polymer electrolytes in fuel cells [J].
Aoki, M ;
Uchida, H ;
Watanabe, M .
ELECTROCHEMISTRY COMMUNICATIONS, 2005, 7 (12) :1434-1438
[3]   Degradation of polymer electrolyte membranes [J].
Collier, Amanda ;
Wang, Haijiang ;
Yuan, Xiao Zi ;
Zhang, Jiujun ;
Wilkinson, David P. .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2006, 31 (13) :1838-1854
[4]   Fuzzy-clustering durability diagnosis of polymer electrolyte fuel cells dedicated to transportation applications [J].
Hissel, Daniel ;
Candusso, Denis ;
Harel, Fabien .
IEEE TRANSACTIONS ON VEHICULAR TECHNOLOGY, 2007, 56 (05) :2414-2420
[5]   Description of gasket failure in a 7 cell PEMFC stack [J].
Husar, Attila ;
Serra, Maria ;
Kunusch, Cristian .
JOURNAL OF POWER SOURCES, 2007, 169 (01) :85-91
[6]   Gas crossover and membrane degradation in polymer electrolyte fuel cells [J].
Inaba, Minoru ;
Kinumoto, Taro ;
Kiriake, Masayuki ;
Umebayashi, Ryota ;
Tasaka, Akimasa ;
Ogumi, Zempachi .
ELECTROCHIMICA ACTA, 2006, 51 (26) :5746-5753
[7]  
LaConti A.B., 2003, HDB FUEL CELLS, V3, P647
[8]   Degradation of elastomeric gasket materials in PEM fuel cells [J].
Tan, Jinzhu ;
Chao, Y. J. ;
Van Zee, J. W. ;
Lee, W. K. .
MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING, 2007, 445 :669-675
[9]   Diagnosis methods dedicated to the localisation of failed cells within PEMFC stacks [J].
Tian, Guangyu ;
Wasterlain, Sebastien ;
Endichi, Issame ;
Candusso, Denis ;
Harel, Fabien ;
Francois, Xavier ;
Pera, Marie-Cecile ;
Hissel, Daniel ;
Kauffmann, Jean-Marie .
JOURNAL OF POWER SOURCES, 2008, 182 (02) :449-461
[10]  
Wilkinson D.P., 2003, HDB FUEL CELLS FUNDA, P611