Methane and nitrous oxide annual emissions from an old eutrophic temperate reservoir

被引:45
作者
Descloux, S. [1 ]
Chanudet, V. [1 ]
Serca, D. [2 ]
Guerin, F. [3 ,4 ]
机构
[1] EDF, Hydro Engn Ctr, Environm & Soc Dept, F-73373 Le Bourget Du Lac, France
[2] Univ Toulouse, Lab Aerol, CNRS, UPS,UMR5560, 14 Av Edouard Belin, F-31400 Toulouse, France
[3] Univ Toulouse, UPS GET, 14 Ave E Belin, F-31400 Toulouse, France
[4] Inst Rech Dev, UR 234, GET, 14 Ave E Belin, F-31400 Toulouse, France
关键词
Methane; Nitrous oxide; Diffusion; Ebullition; Degassing; Eguzon reservoir; GREENHOUSE-GAS EMISSIONS; HYDROELECTRIC RESERVOIRS; CH4; EMISSIONS; SPATIAL HETEROGENEITY; TRANSFER VELOCITIES; TROPICAL RESERVOIR; DIFFUSIVE METHANE; PETIT SAUT; WATER; CARBON;
D O I
10.1016/j.scitotenv.2017.04.066
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Two greenhouse gases-methane (CH4) and nitrous oxide (N2O) - were monitored monthly during one year (2011) at the Eguzon Reservoir in France. The objective of the study was to quantify for the first time in a temperate area the total emissions of these gases through the main emission pathways (diffusion and bubbling from the reservoir, degassing and downstream diffusion). The reservoir was impounded in 1926 and had, in 2011, a eutrophic status promoting high organic matter degradation and nitrification-denitrification, all favouring CH4 and N2O production. CH4 and N2O emissions were dominated by diffusion from the reservoir surface (respectively 78.0% and 92.3%). Ebullition was only observed for CH4 and accounted for 14.0% of total CH4 emissions. Downstream degassing and diffusion represented 8.1% of the total CH4 emissions and 7.7% of the total N2O emissions. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:959 / 972
页数:14
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