Hydrothermal synthesis of nitrogen-doped carbon dots as a sensitive fluorescent probe for the rapid, selective determination of Hg2+

被引:13
作者
Zhang, Yong [1 ]
Jing, Na [1 ]
Zhang, Junqiu [1 ]
Wang, Yingte [1 ]
机构
[1] Shanxi Univ, Sch Chem & Chem Engn, Taiyuan, Shanxi, Peoples R China
关键词
Hydrothermal synthesis; nitrogen-doped carbon dots; ammonium citrate; urea; Hg2+; GRAPHENE QUANTUM DOTS; TURN-ON DETECTION; GREEN SYNTHESIS; MERCURY(II) IONS; NANOPARTICLES; NANODOTS; ELECTRODES; SPECIATION; ROUTE; CELLS;
D O I
10.1080/03067319.2017.1355969
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
In the present work, a green synthetic method for producing nitrogen-doped carbon dots (NCDs) by using ammonium citrate and urea is introduced. The obtained NCDs were characterised by transmission electron microscopy, Fourier transform infrared spectra, UV-vis absorption and fluorescence spectra. The results showed that the prepared NCDs were spherical with a size of about 3.5 nm, emitting strong and stable blue fluorescence when excited at 352 nm. It was noting that the NCDs enable sensitive and selective determination of Hg2+ in tap water with a linear range of 0.01-5 mg L-1 based on a possible charge transfer process. The detection limit was 9.4 mu g L-1.
引用
收藏
页码:841 / 853
页数:13
相关论文
共 45 条
  • [1] Preparation of Graphene Quantum Dots from Pyrolyzed Alginate
    Atienzar, Pedro
    Primo, Ana
    Lavorato, Cristina
    Molinari, Raffaele
    Garcia, Hermenegildo
    [J]. LANGMUIR, 2013, 29 (20) : 6141 - 6146
  • [2] Luminescent Carbon Nanodots: Emergent Nanolights
    Baker, Sheila N.
    Baker, Gary A.
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (38) : 6726 - 6744
  • [3] Isolation and characterization of fluorescent nanoparticles from pristine and oxidized electric arc-produced single-walled carbon nanotubes
    Bottini, M
    Balasubramanian, C
    Dawson, MI
    Bergamaschi, A
    Bellucci, S
    Mustelin, T
    [J]. JOURNAL OF PHYSICAL CHEMISTRY B, 2006, 110 (02) : 831 - 836
  • [4] INFLUENCE OF CHEMICAL-SPECIES ON THE DETERMINATION OF MERCURY IN A BIOLOGICAL MATRIX (COD MUSCLE) USING INDUCTIVELY COUPLED PLASMA MASS-SPECTROMETRY
    CAMPBELL, MJ
    VERMEIR, G
    DAMS, R
    QUEVAUVILLER, P
    [J]. JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY, 1992, 7 (04) : 617 - 621
  • [5] A green and facile approach for the synthesis of water soluble fluorescent carbon dots from banana juice
    De, Bibekananda
    Karak, Niranjan
    [J]. RSC ADVANCES, 2013, 3 (22): : 8286 - 8290
  • [6] Effect of carbon-dots modification on the structure and photocatalytic activity of g-C3N4
    Fang, Shun
    Xia, Yang
    Lv, Kangle
    Li, Qin
    Sun, Jie
    Li, Mei
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2016, 185 : 225 - 232
  • [7] Carbon quantum dot-based nanoprobes for metal ion detection
    Gao, Xiaohui
    Du, Cheng
    Zhuang, Zhihua
    Chen, Wei
    [J]. JOURNAL OF MATERIALS CHEMISTRY C, 2016, 4 (29) : 6927 - 6945
  • [8] One-pot synthesis of carbon nanodots for fluorescence turn-on detection of Ag+ based on the Ag+-induced enhancement of fluorescence
    Gao, Xiaohui
    Lu, Yizhong
    Zhang, Ruizhong
    He, Shuijian
    Ju, Jian
    Liu, Minmin
    Li, Lei
    Chen, Wei
    [J]. JOURNAL OF MATERIALS CHEMISTRY C, 2015, 3 (10) : 2302 - 2309
  • [9] A fluorescent probe based on N-doped carbon dots for highly sensitive detection of Hg2+ in aqueous solutions
    Gao, Zhi-hao
    Lin, Zheng-zhong
    Chen, Xiao-mei
    Zhong, Hui-ping
    Huang, Zhi-yong
    [J]. ANALYTICAL METHODS, 2016, 8 (10) : 2297 - 2304
  • [10] Highly selective and sensitive preconcentration of mercury ion and determination by cold vapor atomic absorption spectroscopy
    Ghaedi, M
    Fathi, MR
    Shokrollahi, A
    Shajarat, F
    [J]. ANALYTICAL LETTERS, 2006, 39 (06) : 1171 - 1185