Photoelectrochemical detection of tetracycline with exceptional speediness, ultralow detection limit, and high selectivity

被引:51
作者
Chen, Feng-Zao [1 ,2 ]
Gao, Yuan [3 ]
Li, Yu-Jun [2 ]
Li, Wei [2 ]
Wu, Xiao-Yu [1 ]
Han, De-Man [1 ,2 ]
Zhao, Wei-Wei [3 ]
机构
[1] Taizhou Univ, Taizhou Univ Hosp, Taizhou Cent Hosp, Dept Clin Lab, Jiaojiang 318000, Peoples R China
[2] Taizhou Univ, Sch Pharmaceut Chem & Mat Engn, Jiaojiang 318000, Peoples R China
[3] Nanjing Univ, Sch Chem & Chem Engn, State Key Lab Analyt Chem Life Sci, Nanjing 210023, Peoples R China
基金
中国国家自然科学基金;
关键词
Photoelectrochemical Sensor; MOF; Tetracycline; Rapid Response; High Sensitivity; ANTIBIOTICS; MILK;
D O I
10.1016/j.snb.2022.131651
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Metal-organic frameworks (MOFs) with unique physicochemical properties have found increasing applications in various fields including photoelectrochemical (PEC) sensors. This work describes a high-performance MOF-based PEC sensor towards tetracycline (TET), a kind of stable broad-spectrum antibiotics. Specifically, zeolitic imidazolate framework-8 (ZIF-8), on top of ZnIn2S4 nanosheets (ZIS)/fluorine-doped tin oxide (FTO), could interact with TET in a rapid and selective manner, causing the substantial reduction of the photocurrent signal. In TET detection, this sensor could quickly respond to TET with ultralow detection limit of 0.1 pM. In addition to a new TET sensor, this work is expected to inspire more interest in the development of advanced MOF-based PEC sensors.
引用
收藏
页数:5
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