Radiocesium in Ponds in the Near Zone of Fukushima Dai-ichi NPP

被引:19
作者
Konoplev, A. V. [1 ]
Wakiyama, Y. [1 ]
Wada, T. [1 ]
Golosov, V. N. [2 ]
Nanba, K. [1 ]
Takase, T. [1 ]
机构
[1] Fukushima Univ, Environm Radioact Inst, Fukushima 9601296, Japan
[2] Moscow MV Lomonosov State Univ, Fac Geog, Moscow 119991, Russia
基金
日本学术振兴会;
关键词
Fukushima; radiocesium; ponds; solution; particulate matter; POWER-PLANT ACCIDENT; NUCLEAR ACCIDENT; LAKE-SEDIMENTS; WATER; CONTAMINATION; SOILS;
D O I
10.1134/S0097807818040139
中图分类号
TV21 [水资源调查与水利规划];
学科分类号
081501 ;
摘要
The article presents the results of studying radiocesium concentration and distribution between dissolved and particulate forms in ponds in the near zone of Fukushima Dai-ichi NPP NPP after the 2011 accident. The total concentration of Cs-137 in pond water and its variations are shown to be largely governed by the concentration of particulate matter being as high as 68 Bq/L, compared with 5 Bq/L in solution. The values of the distribution coefficient K-d in the ponds are similar to those in rivers and in large flow-through lakes in the accidentally polluted zone at Fukushima Dai-ichi NPP. The contributions of the main competing ions K+ and NH4+ to radiocesium desorption from solid particles into solution were similar for the ponds; however, their relative effect on dissolved radiocesium concentration varied over time because of variations in ammonium concentration.
引用
收藏
页码:589 / 597
页数:9
相关论文
共 27 条
[11]   Behavior of accidentally released radiocesium in soil-water environment: Looking at Fukushima from a Chernobyl perspective [J].
Konoplev, A. ;
Golosov, V. ;
Laptev, G. ;
Nanba, K. ;
Onda, Y. ;
Takase, T. ;
Wakiyama, Y. ;
Yoshimura, K. .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 2016, 151 :568-578
[12]   Comparative study of 137Cs partitioning between solid and liquid phases in Lakes Constance, Lugano and Vorsee [J].
Konoplev, A ;
Kaminski, S ;
Klemt, E ;
Konopleva, I ;
Miller, R ;
Zibold, G .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 2002, 58 (01) :1-11
[13]   Vertical distribution of radiocesium in soils of the area affected by the Fukushima Dai-ichi nuclear power plant accident [J].
Konoplev, A. V. ;
Golosov, V. N. ;
Yoschenko, V. I. ;
Nanba, K. ;
Onda, Y. ;
Takase, T. ;
Wakiyama, Y. .
EURASIAN SOIL SCIENCE, 2016, 49 (05) :570-580
[14]  
Konoplev A.V., 1992, SOV MTEOROL HYDROL, V1, P35
[15]  
Konoplev A.V., 1998, METEOROL GIDROL, P78
[16]  
Konoplev A.V., 1999, GEOCHEM INTERNAT, V37, P177
[17]  
Konoplev A.V, 1998, THESIS
[18]  
Konoplev A. V, 2015, RADIOKHIMIYA, V57, P471
[19]  
Moiseenko T.I., 2009, Vodnaya Ekotoksikologiya: Teoreticheskie i Prikladnye Aspekty
[20]  
Moiseenko T.I., 2005, WATER RESOUR, V32, P163