Radiocesium in Ponds in the Near Zone of Fukushima Dai-ichi NPP

被引:19
作者
Konoplev, A. V. [1 ]
Wakiyama, Y. [1 ]
Wada, T. [1 ]
Golosov, V. N. [2 ]
Nanba, K. [1 ]
Takase, T. [1 ]
机构
[1] Fukushima Univ, Environm Radioact Inst, Fukushima 9601296, Japan
[2] Moscow MV Lomonosov State Univ, Fac Geog, Moscow 119991, Russia
基金
日本学术振兴会;
关键词
Fukushima; radiocesium; ponds; solution; particulate matter; POWER-PLANT ACCIDENT; NUCLEAR ACCIDENT; LAKE-SEDIMENTS; WATER; CONTAMINATION; SOILS;
D O I
10.1134/S0097807818040139
中图分类号
TV21 [水资源调查与水利规划];
学科分类号
081501 ;
摘要
The article presents the results of studying radiocesium concentration and distribution between dissolved and particulate forms in ponds in the near zone of Fukushima Dai-ichi NPP NPP after the 2011 accident. The total concentration of Cs-137 in pond water and its variations are shown to be largely governed by the concentration of particulate matter being as high as 68 Bq/L, compared with 5 Bq/L in solution. The values of the distribution coefficient K-d in the ponds are similar to those in rivers and in large flow-through lakes in the accidentally polluted zone at Fukushima Dai-ichi NPP. The contributions of the main competing ions K+ and NH4+ to radiocesium desorption from solid particles into solution were similar for the ponds; however, their relative effect on dissolved radiocesium concentration varied over time because of variations in ammonium concentration.
引用
收藏
页码:589 / 597
页数:9
相关论文
共 27 条
[1]   Detection of Uranium and Chemical State Analysis of Individual Radioactive Microparticles Emitted from the Fukushirna Nuclear Accident Using Multiple Synchrotron Radiation X-ray Analyses [J].
Abe, Yoshinari ;
Iizawa, Yushin ;
Terada, Yasuko ;
Adachi, Kouji ;
Igarashi, Yasuhito ;
Nakai, Izumi .
ANALYTICAL CHEMISTRY, 2014, 86 (17) :8521-8525
[2]   Emission of spherical cesium-bearing particles from an early stage of the Fukushima nuclear accident [J].
Adachi, Kouji ;
Kajino, Mizuo ;
Zaizen, Yuji ;
Igarashi, Yasuhito .
SCIENTIFIC REPORTS, 2013, 3
[3]  
[Anonymous], 2012, RES I 5 AIRB MON SUR
[4]   MOBILIZATION OF RADIOCESIUM IN PORE WATER OF LAKE-SEDIMENTS [J].
COMANS, RNJ ;
MIDDELBURG, JJ ;
ZONDERHUIS, J ;
WOITTIEZ, JRW ;
DELANGE, GJ ;
DAS, HA ;
VANDERWEIJDEN, CH .
NATURE, 1989, 339 (6223) :367-369
[5]   QUANTITATIVE-ANALYSIS OF RADIOCESIUM RETENTION IN SOILS [J].
CREMERS, A ;
ELSEN, A ;
DEPRETER, P ;
MAES, A .
NATURE, 1988, 335 (6187) :247-249
[6]   Measuring the specific caesium sorption capacity of soils, sediments and clay minerals [J].
de Koning, A. ;
Konoplev, A. V. ;
Comans, R. N. J. .
APPLIED GEOCHEMISTRY, 2007, 22 (01) :219-229
[7]  
De Preter, 1990, THESIS
[8]   Radiocesium contamination of lake sediments and fish following the Fukushima nuclear accident and their partition coefficient [J].
Fukushima, Takehiko ;
Arai, Hiroyuki .
INLAND WATERS, 2014, 4 (02) :204-214
[9]   2011 Fukushima Dai-ichi nuclear power plant accident: summary of regional radioactive deposition monitoring results [J].
Hirose, Katsumi .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 2012, 111 :13-17
[10]   Sulfate Aerosol as a Potential Transport Medium of Radiocesium from the Fukushima Nuclear Accident [J].
Kaneyasu, Naoki ;
Ohashi, Hideo ;
Suzuki, Fumie ;
Okuda, Tomoaki ;
Ikemori, Fumikazu .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2012, 46 (11) :5720-5726