Shift of the Optimum Binding Energy at Higher Rates of Catalysis

被引:76
作者
Ooka, Hideshi [1 ]
Nakamura, Ryuhei [1 ,2 ]
机构
[1] RIKEN, CSRS, Biofunct Catalyst Res Team, 2-1 Hirosawa, Wako, Saitama 3510198, Japan
[2] Tokyo Inst Technol, ELSI, Meguro Ku, 2-12-IE-1 Ookayama, Tokyo 1528550, Japan
关键词
ELECTROCHEMICAL HYDROGEN OXIDATION; EVOLUTION ELECTROCATALYSIS; REDUCTION; UNIVERSALITY; ADSORPTION; DESIGN;
D O I
10.1021/acs.jpclett.9b01796
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The binding energy between the catalyst and the reactant is considered to be the primary descriptor of catalytic activity. Therefore, identifying the optimum binding energy that would yield maximum activity is fundamentally important for the development of efficient catalysts. Here, we show analytically how the binding energy that maximizes the activity at large reaction rates, i.e., the operating conditions of catalysis, may deviate from the traditional understanding obtained near equilibrium. This shift can be on the order of 0.5 eV, which is easily sufficient for the optimum material to change. This binding energy shift is consistent with experimental observations in the literature, suggesting that a reinvestigation of materials previously considered to be inactive may be necessary.
引用
收藏
页码:6706 / 6713
页数:15
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