All-Optical Three-Dimensional Electron Momentum Imaging

被引:6
作者
Orunesajo, Emmanuel [1 ]
Basnayake, Gihan [1 ]
Ranathunga, Yasashri [1 ]
Stewart, Gabriel [1 ]
Heathcote, David [2 ]
Vallance, Claire [2 ]
Lee, Suk Kyoung [1 ]
Li, Wen [1 ]
机构
[1] Wayne State Univ, Dept Chem, Detroit, MI 48202 USA
[2] Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England
基金
英国工程与自然科学研究理事会;
关键词
ION;
D O I
10.1021/acs.jpca.1c03445
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We report a new implementation of three-dimensional ( 3D) momentum imaging for electrons, employing a two-dimensional (2D) imaging detector and a silicon photomultiplier tube (siPMT). To achieve the necessary time resolution for 3D electron imaging, a poly(p-phenylene)-dye-based fast scintillator (Exalite 404) was used in the imaging detector instead of conventional phosphors. The system demonstrated an electron time-of-flight resolution comparable with that of electrical MCP pick-off (tens of picoseconds), while achieving an unprecedented dead time reduction (similar to 0.48 ns) when detecting two electrons.
引用
收藏
页码:5220 / 5225
页数:6
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