Manganese(III,IV) and manganese(III) oxide clusters trapped by copper(II) complexes

被引：28
|
作者：
Yamashita, Satoshi
Shiga, Takuya
Kurashina, Masashi
Nihei, Masayuki
Nojiri, Hiroyuki
Sawa, Hiroshi
Kakiuchi, Toru
Oshio, Hiroki
机构：
[1] Univ Tsukuba, Dept Chem, Grad Sch Pure & Appl Sci, Tsukuba, Ibaraki 3058571, Japan
[2] Tohoku Univ, Mat Res Inst, Aoba Ku, Sendai, Miyagi, Japan
[3] High Energy Accelerator Res Org, Inst Mat Res Sci, Tsukuba, Ibaraki 3050801, Japan
来源：
INORGANIC CHEMISTRY | 2007年 / 46卷 / 10期
关键词：
D O I：
10.1021/ic062258h
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
Reactions of quinquedentate Schiff base ligands with Mn and Cu ions afforded icosa- and hexadecanuclear mixed-metal clusters in which dinuclear Cu-II complexes trapped oxo-bridged [(Mn8Mn4O12)-Mn-III-O-IV] and [(Mn6O6)-O-III] cores, respectively. Maximum entropy method analysis for synchrotron X-ray diffraction data was used to determine the oxidation states of the Mn ions.
引用
收藏
页码：3810 / 3812
页数：3
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