Electrodynamical treatment of the electron-hole long-range exchange interaction in semiconductor nanocrystals

被引:16
作者
Goupalov, SV [1 ]
Lavallard, P
Lamouche, G
Citrin, DS
机构
[1] Georgia Inst Technol, Sch Elect & Comp Engn, Atlanta, GA 30332 USA
[2] Russian Acad Sci, AF Ioffe Physicotech Inst, St Petersburg 194021, Russia
[3] Univ Paris 07, Phys Solides Grp, CNRS, UMR 7588, F-75251 Paris 05, France
[4] Univ Paris 06, F-75251 Paris 05, France
[5] Natl Res Council Canada, IMI, Boucherville, PQ J4B 6Y4, Canada
基金
美国国家科学基金会;
关键词
D O I
10.1134/1.1569020
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
We show that the contribution to the fine structure of the ground exciton level in a semiconductor nanocrystal due to the long-range part of the electron-hole exchange interaction can be equivalently described as arising from the mechanical exciton interaction with the exciton-induced macroscopic longitudinal electric field. Particular cases of nanocrystals with cubic and wurtzite crystal lattice in the strong confinement regime are studied taking into account the complex structure of the valence band. A simplified model accounting for the exciton ground-level splitting and exploiting an effective local scalar susceptibility is established. (C) 2003 MAIK "Nauka / Interperiodica".
引用
收藏
页码:768 / 781
页数:14
相关论文
共 36 条
  • [21] Anisotropic exchange splitting of excitonic levels in small quantum systems
    Goupalov, SV
    Ivchenko, EL
    Kavokin, AV
    [J]. SUPERLATTICES AND MICROSTRUCTURES, 1998, 23 (06) : 1205 - 1209
  • [22] The fine structure of excitonic levels in CdSe nanocrystals
    Gupalov, SV
    Ivchenko, EL
    [J]. PHYSICS OF THE SOLID STATE, 2000, 42 (11) : 2030 - 2038
  • [23] Ivchenko E. L., 1997, Superlattices and Other Heterostructures: Symmetry and Optical Phenomena
  • [24] Landau L. D., 1960, ELECTRODYNAMICS CONT
  • [25] Influence of surrounding dielectrics on the spontaneous emission of sulforhodamine B molecules
    Lavallard, P
    Rosenbauer, M
    Gacoin, T
    [J]. PHYSICAL REVIEW A, 1996, 54 (06): : 5450 - 5453
  • [26] Excitons in nanocrystals
    Lavallard, P
    [J]. JOURNAL OF CRYSTAL GROWTH, 1998, 184 : 352 - 359
  • [27] LAVALLARD P, IN PRESS
  • [28] Electron-hole correlations in semiconductor quantum dots with tight-binding wave functions -: art. no. 195318
    Lee, S
    Jönsson, L
    Wilkins, JW
    Bryant, GW
    Klimeck, G
    [J]. PHYSICAL REVIEW B, 2001, 63 (19)
  • [29] OBSERVATION OF THE DARK EXCITON IN CDSE QUANTUM DOTS
    NIRMAL, M
    NORRIS, DJ
    KUNO, M
    BAWENDI, MG
    EFROS, AL
    ROSEN, M
    [J]. PHYSICAL REVIEW LETTERS, 1995, 75 (20) : 3728 - 3731
  • [30] Size dependence of exciton fine structure in CdSe quantum dots
    Norris, DJ
    Efros, AL
    Rosen, M
    Bawendi, MG
    [J]. PHYSICAL REVIEW B, 1996, 53 (24): : 16347 - 16354