Experiments and fully transient coupled CFD-PBM 3D flow simulations of disperse liquid-liquid flow in a baffled stirred tank

Liquid-liquid disperse multiphase flow in a baffled tank stirred by a Rushton turbine is investigated by experiments and 3D simulations for different impeller speeds and volume fractions. Droplet size distributions are experimentally measured with an inline shadowgraphic probe and compared with fully transient coupled CFD-PBM simulations using the Eulerian multi-fluid framework, the inhomogeneous Multiple Size Group approach and a statistical turbulence model. The simulation model is assessed by a variation of size class and velocity group numbers, grid resolution and simulation domain extent. The model parameters for the breakup and coalescence kernels are fitted to match the measured droplet size distribution at a selected operation point. A subsequent application to different operation points shows that experimental droplet size trends are captured, albeit aside from the fitting point, deviations to data increase. The resulting droplet size distribution is analyzed by an assessment of the turbulent mixing, breakup and coalescence time scales. (c) 2022 Elsevier Ltd. All rights reserved.