Creep and aging of hard-sphere glasses under constant stress

被引:28
作者
Ballesta, P. [1 ,2 ]
Petekidis, G. [2 ,3 ]
机构
[1] Univ Porto, Fac Engn, CEFT, Dept Engn Quim, Rua Dr Roberto Frias, P-4200465 Oporto, Portugal
[2] IESL FORTH, POB 1527, Iraklion 71110, Crete, Greece
[3] Univ Crete, Dept Mat Sci & Technol, Iraklion, Greece
关键词
TEMPORALLY HETEROGENEOUS DYNAMICS; COLLOIDAL GLASSES; AMORPHOUS MATERIALS; LIGHT-SCATTERING; SLOW DYNAMICS; RHEOLOGY; FLOW; BEHAVIOR; MODEL; SHEAR;
D O I
10.1103/PhysRevE.93.042613
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We investigate the aging behavior of glassy suspensions of nearly hard-sphere colloids submitted to a constant shear stress. For low stresses, below the yield stress, the system is subject to creep motion. As the sample ages, the shear rate exhibits a power-law decrease with time with exponents that depend on the sample age. We use a combination of rheological experiments with time-resolved photon correlation spectroscopy to investigate the time evolution of the sample dynamics under shear on various time and length scales. Long-time light-scattering experiments reveal the occurrence of microscopic rearrangement events that are linked with the macroscopic strain deformation of the sample. Dynamic time sweep experiments indicate that while the internal microscopic dynamics slow down continuously with waiting time, the storage and loss moduli are almost constant after a fast, weak decrease, resembling the behavior of quenched systems with partially frozen-in stresses.
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页数:10
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