Modeling of alpha mass-efficiency curve

We present a model for efficiency of a detector counting gross a radioactivity from both thin and thick samples, corresponding to low and high sample masses in the counting planchette. The model includes self-absorption of a particles in the sample, energy loss in the absorber, range straggling, as well as detector edge effects. The surface roughness of the sample is treated in terms of fractal geometry. The model reveals a linear dependence of the detector efficiency on the sample mass, for low masses, as well as a power-law dependence for high masses. It is, therefore, named the linear-power-law (LPL) model. In addition, we consider an empirical power-law (EPL) curve, and an exponential (EXP) curve. A comparison is made of the LPL, EPL, and EXP fits to the experimental a mass-efficiency data from gas-proportional detectors for selected radionuclides: U-238, Th-230, Pu-239, Am-241, and Cm-244. Based on this comparison, we recommend working equations for fitting mass-efficiency data. Measurement of a radioactivity from a thick sample can determine the fractal dimension of its surface. (C) 2004 Elsevier B.V. All rights reserved.