The role of substrate electrons in the wetting of a metal surface

被引:40
作者
Schiros, T. [1 ,2 ]
Takahashi, O. [2 ,3 ]
Andersson, K. J. [4 ]
Ostrom, H. [2 ]
Pettersson, L. G. M. [2 ]
Nilsson, A. [1 ,2 ,5 ]
Ogasawara, H. [1 ,2 ,5 ]
机构
[1] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA
[2] Stockholm Univ, AlbaNova Univ Ctr, FYSIKUM, S-10691 Stockholm, Sweden
[3] Hiroshima Univ, Grad Sch Sci, Dept Chem, Higashihiroshima 7398526, Japan
[4] Tech Univ Denmark, CINF, Dept Phys, DK-2800 Lyngby, Denmark
[5] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA
基金
美国国家科学基金会;
关键词
bonds (chemical); copper; crystal field interactions; platinum; surface states; surface structure; water; wetting; DENSITY-FUNCTIONAL THEORY; AB-INITIO; WATER-ADSORPTION; SOLID-SURFACES; WORK-FUNCTION; ICE; ANISOTROPY; CU(110); OXYGEN; MODEL;
D O I
10.1063/1.3292681
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We address how the electronic and geometric structures of metal surfaces determine water-metal bonding by affecting the balance between Pauli repulsion and electrostatic attraction. We show how the rigid d-electrons and the softer s-electrons utilize different mechanisms for the redistribution of charge that enables surface wetting. On open d-shell Pt(111), the ligand field of water alters the distribution of metal d-electrons to reduce the repulsion. The closed-shell Cu d(10) configuration of isostructural Cu(111), however, does not afford this mechanism, resulting in a hydrophobic surface and three-dimensional ice cluster formation. On the geometrically corrugated Cu(110) surface, however, charge depletion involving the mobile sp-electrons at atomic rows reduces the exchange repulsion sufficiently such that formation of a two-dimensional wetting layer is still favored in spite of the d(10) electronic configuration.
引用
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页数:9
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