Low-energy positron collisions with water: elastic and rotationally inelastic scattering

被引:38
作者
Baluja, K. L. [1 ]
Zhang, Rui
Franz, Jan
Tennyson, Jonathan
机构
[1] Univ Delhi, Dept Phys & Astrophys, Delhi 110007, India
[2] UCL, Dept Phys & Astron, London WC1E 6BT, England
基金
英国工程与自然科学研究理事会;
关键词
D O I
10.1088/0953-4075/40/17/018
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Differential, integral and momentum transfer cross sections for the vibrationally elastic and rotationally inelastic scattering of positrons from water at low collision energy ( E <= 10 eV) are reported. Several models within the R-matrix method are used to compute the body-fixed T-matrices, while the scattering calculations are performed within the fixed-nuclei approximation corrected with the standard Born-closure formula. These calculations are compared with experimental results for elastic scattering, and the best model gives reasonable agreement with the most recent measurements (Zecca et al 2006 J. Phys. B: At. Mol. Opt. Phys. 39 1597) but not with some earlier studies. The relative contribution of the rotationally inelastic processes is investigated and comparisons are made with the equivalent electron scattering cross sections.
引用
收藏
页码:3515 / 3524
页数:10
相关论文
共 35 条
[1]   METHODS AND PROGRAMS IN COLLISIONS OF POSITRONS WITH ATOMS AND MOLECULES [J].
ARMOUR, EAG ;
HUMBERSTON, JW .
PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 1991, 204 (02) :165-251
[2]   Electron collisions with ClO using the R-matrix method [J].
Baluja, KL ;
Mason, NJ ;
Morgan, LA ;
Tennyson, J .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2000, 33 (20) :L677-L684
[3]   Positronium- and positron-H2O total cross sections [J].
Beale, J ;
Armitage, S ;
Laricchia, G .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2006, 39 (06) :1337-1344
[4]   Elastic electron scattering from water vapor at backward angles [J].
Cho, H ;
Lee, HS ;
Park, YS .
RADIATION PHYSICS AND CHEMISTRY, 2003, 68 (1-2) :115-120
[5]   On equilibrium structures of the water molecule -: art. no. 214305 [J].
Császár, AG ;
Czakó, G ;
Furtenbacher, T ;
Tennyson, J ;
Szalay, V ;
Shirin, SV ;
Zobov, NF ;
Polyansky, OL .
JOURNAL OF CHEMICAL PHYSICS, 2005, 122 (21)
[6]   Rotational excitation of H2O by cold electrons [J].
Curik, R. ;
Ziesel, J. P. ;
Jones, N. C. ;
Field, T. A. ;
Field, D. .
PHYSICAL REVIEW LETTERS, 2006, 97 (12)
[7]   POSITRON-HF COLLISIONS - PREDICTION OF A WEAKLY BOUND-STATE [J].
DANBY, G ;
TENNYSON, J .
PHYSICAL REVIEW LETTERS, 1988, 61 (24) :2737-2739
[8]  
DANBY G, 1990, J PHYS B-AT MOL OPT, V23, P2471
[9]   DIFFERENTIAL CROSS-SECTIONS FOR ELASTIC POSITRON-H-2 COLLISIONS USING THE R-MATRIX METHOD [J].
DANBY, G ;
TENNYSON, J .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1990, 23 (06) :1005-1016
[10]   R-MATRIX CALCULATIONS OF VIBRATIONALLY RESOLVED POSITRON N2 SCATTERING CROSS-SECTIONS [J].
DANBY, G ;
TENNYSON, J .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1991, 24 (15) :3517-3529