Free-induction decay and envelope modulations in a narrowed nuclear spin bath

被引:63
作者
Coish, W. A. [1 ,2 ,3 ]
Fischer, Jan [4 ]
Loss, Daniel [3 ,4 ]
机构
[1] Univ Waterloo, Inst Quantum Comp, Waterloo, ON N2L 3G1, Canada
[2] Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada
[3] UCSB, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA
[4] Univ Basel, Dept Phys, CH-4056 Basel, Switzerland
基金
美国国家科学基金会; 加拿大自然科学与工程研究理事会;
关键词
SINGLE-ELECTRON SPIN; COUPLED ELECTRON; QUANTUM; RESONANCE; DYNAMICS; LOCKING; DIFFUSION; FIELD;
D O I
10.1103/PhysRevB.81.165315
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We evaluate free-induction decay for the transverse components of a localized electron spin coupled to a bath of nuclear spins via the Fermi-contact hyperfine interaction. Our perturbative treatment is valid for special (narrowed) bath initial conditions and when the Zeeman energy of the electron b exceeds the total hyperfine coupling constant A: b > A. Using one unified and systematic method, we recover previous results reported at short and long times using different techniques. We find an unexpected modulation of the free-induction-decay envelope, which is present even for a purely isotropic hyperfine interaction without spin echoes and for a single nuclear species. We give subleading corrections to the decoherence rate, and show that, in general, the decoherence rate has a nonmonotonic dependence on electron Zeeman splitting, leading to a pronounced maximum. These results illustrate the limitations of methods that make use of leading-order effective Hamiltonians and re-exponentiation of short-time expansions for a strongly interacting system with non-Markovian (history-dependent) dynamics.
引用
收藏
页数:13
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