Oxide Semiconductor Phototransistor with Organolead Trihalide Perovskite Light Absorber

被引:68
作者
Du, Songnan [1 ]
Li, Gongtan [2 ]
Cao, Xuhong [2 ]
Wang, Yan [1 ]
Lu, Huiling [1 ]
Zhang, Shengdong [1 ]
Liu, Chuan [2 ]
Zhou, Hang [1 ]
机构
[1] Peking Univ, Shenzhen Grad Sch, Shenzhen Key Lab Thin Film Transistor & Adv Displ, Shenzhen 518055, Peoples R China
[2] Sun Yat Sen Univ, State Key Lab Optoelect Mat & Technol, Guangdong Prov Key Lab Display Mat & Technol, Sch Elect & Informat Technol, Guangzhou 510275, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
METHYLAMMONIUM LEAD IODIDE; SOLAR-CELL; PERSISTENT PHOTOCONDUCTIVITY; HALIDE PEROVSKITE; PHOTODETECTORS; FABRICATION; ARRAYS;
D O I
10.1002/aelm.201600325
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
A hybrid phototransistor is developed with solution-processed organolead trihalide perovskite (MAPbI(3)) capping indium gallium zinc oxide (IGZO), which well fuses the properties of the two materials in sensitive photodetecting and high-mobility charge transporting, respectively. The MAPbI(3)-capped IGZO phototransistor demonstrates excellent responsivities of over 25 mA W-1 for lights with photon energies above the bandgap of perovskite light absorber. Besides the high sensitivity to light in both ultraviolet and visible regions, hybrid phototransistor maintains a fair on/off ratio of over 106 in the dark, and a field effect mobility of 12.9 cm(2) V-1 s(-1). The perovskite light absorber also obviates the long-standing problem for metal oxide phototransistor, the persistent photoconductivity behavior. Furthermore, fast transient response has been achieved by showing rise-time and fall-time within tens of milliseconds. The newly developed device opens variable optic-electric sensing applications for the integrated oxide-perovskite hybrid phototransistors.
引用
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页数:6
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