Enhancing Magnetic Light Emission with All-Dielectric Optical Nanoantennas

被引:78
作者
Sanz-Paz, Maria [1 ]
Ernandes, Cyrine [2 ,3 ]
Esparza, Juan Uriel [2 ]
Burr, Geoffrey W. [4 ]
van Hulst, Niek F. [1 ,5 ]
Maitre, Agnes [2 ]
Aigouy, Lionel [3 ]
Gacoin, Thierry [7 ]
Bonod, Nicolas [6 ]
Garcia-Parajo, Maria F. [1 ,5 ]
Bidault, Sebastien [8 ]
Mivelle, Mathieu [1 ,2 ]
机构
[1] Barcelona Inst Sci & Technol, ICFO Inst Ciencies Foton, Barcelona 08860, Spain
[2] Sorbonne Univ, CNRS, Inst NanoSci Paris, UMR 7588, F-75005 Paris, France
[3] ESPCI Paristech, CNRS, Lab Phys & Etud Mat, F-75005 Paris, France
[4] IBM Corp, Almaden Res Ctr, 650 Harry Rd, San Jose, CA 95120 USA
[5] ICREA, Pg Lluis Co 23, Barcelona 08010, Spain
[6] Aix Marseille Univ, CNRS, Cent Marseille, Inst Fresnel, Marseille, France
[7] Ecole Polytech, Lab Phys Matiere Condensee, Route Saclay, F-91128 Palaiseau, France
[8] PSL Res Univ, ESPCI Paris, CNRS, Inst Langevin, F-75005 Paris, France
关键词
Dielectric and plasmonic nanoantennas; magnetic and electric LDOS; magnetic dipoles; magnetic light; near-field optical microscopy; DIPOLE EMISSION; ELECTRIC-DIPOLE; ANTENNAS; FIELD; TRANSITIONS; RESONANCES; SURFACE; MODES;
D O I
10.1021/acs.nanolett.8b00548
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Electric and magnetic optical fields carry the same amount of energy. Nevertheless, the efficiency with which matter interacts with electric optical fields is commonly accepted to be at least 4 orders of magnitude higher than with magnetic optical fields. Here, we experimentally demonstrate that properly designed photonic nanoantennas can selectively manipulate the magnetic versus electric emission of luminescent nanocrystals. In particular, we show selective enhancement of magnetic emission from trivalent europium-doped nanoparticles in the vicinity of a nanoantenna tailored to exhibit a magnetic resonance. Specifically, by controlling the spatial coupling between emitters and an individual nanoresonator located at the edge of a near-field optical scanning tip, we record with nanoscale precision local distributions of both magnetic and electric radiative local densities of states (LDOS). The map of the radiative LDOS reveals the modification of both the magnetic and electric quantum environments induced by the presence of the nanoantenna. This manipulation and enhancement of magnetic light-matter interaction by means of nanoantennas opens up new possibilities for the research fields of optoelectronics, chiral optics, nonlinear and nano-optics, spintronics, and metamaterials, among others.
引用
收藏
页码:3481 / 3487
页数:7
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