Volatile organic compounds in an e-waste dismantling region: From spatial-seasonal variation to human health impact

被引:41
作者
Chen, Daijin [1 ]
Liu, Ranran [1 ]
Lin, Qinhao [1 ,2 ]
Ma, Shengtao [1 ,2 ]
Li, Guiying [1 ,2 ]
Yu, Yingxin [1 ,2 ]
Zhang, Chaosheng [3 ,4 ]
An, Taicheng [1 ,2 ]
机构
[1] Guangdong Univ Technol, Inst Environm Hlth & Pollut Control, Guangdong Key Lab Environm Catalysis & Hlth Risk, Guangdong Hong Kong Macao Joint Lab Contaminants, Guangzhou 510006, Peoples R China
[2] Guangdong Univ Technol, Sch Environm Sci & Engn, Guangdong Technol Res Ctr Photocatalyt Technol In, Guangzhou Key Lab Environm Catalysis & Pollut Con, Guangzhou 510006, Peoples R China
[3] Natl Univ Ireland, GIS Ctr, Ryan Inst, Galway, Ireland
[4] Natl Univ Ireland, Sch Geog & Archaeol, Galway, Ireland
基金
中国国家自然科学基金;
关键词
Volatile organic compounds; E-waste dismantling region; Seasonal variation; Spatial distribution; Source apportionment; Health risk; AMBIENT MIXING RATIOS; YANGTZE-RIVER DELTA; SOURCE APPORTIONMENT; RISK-ASSESSMENT; POLLUTION PROFILES; ELECTRONIC WASTE; INDUSTRIAL-AREA; OZONE FORMATION; VOCS; EXPOSURE;
D O I
10.1016/j.chemosphere.2021.130022
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Y The dismantling of electrical and electronic waste (e-waste) can release various Volatile organic compounds (VOCs), impacting the surrounding ambient environment. We investigated the spatio-temporal characteristics and health risks of the ambient VOCs emitted in a typical e-waste dismantling region by conducting multi-site sampling campaigns in four seasons. The pollution of benzene, toluene, ethylbenzene, and xylenes (BTEX) in the e-waste dismantling park has relation to e-waste dismantling by seasonal trend analysis. The highest concentrations of most VOCs occurred in winter and autumn, while the lowest levels were observed in summer and spring. The spatial distribution map revealed the e-waste dismantling park to be a hotspot of BTEX, 1,2-dichloropropane (1,2-DCP), and 1,2-dichloroethane (1,2-DCA), while two major residential areas were also the hotspots of BTEX. The e-waste emission source contributed 20.14% to the total VOCs in the e-waste dismantling park, while it was absent in the major residential and rural areas. The cancer risk assessment showed that six VOCs exceeded 1.0 x 10(-6) in the e-waste dismantling park, while only three or four compounds exceeded this risk in other areas. The noncancer risks of all compounds were below the safety threshold. This study supplements the existing knowledge on VOC pollution from e-waste dismantling and expands the research scope of chemical pollution caused by e-waste. (C) 2021 Elsevier Ltd. All rights reserved.
引用
收藏
页数:9
相关论文
共 57 条
  • [1] Environmental Impact of Pyrolysis of Mixed WEEE Plastics Part 1: Experimental Pyrolysis Data
    Alston, Sue M.
    Clark, Allan D.
    Arnold, J. Cris
    Stein, Bridget K.
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2011, 45 (21) : 9380 - 9385
  • [2] Airway Hyperresponsiveness, Inflammation, and Pulmonary Emphysema in Rodent Models Designed to Mimic Exposure to Fuel Oil-Derived Volatile Organic Compounds Encountered during an Experimental Oil Spill
    Amor-Carro, Oscar
    White, Kathryn M.
    Fraga-Iriso, Rebeca
    Marinas-Pardo, Luis A.
    Nunez-Naveira, Laura
    Lema-Costa, Beatriz
    Villarnovo, Marta
    Verea-Hernando, Hector
    Ramos-Barbon, David
    [J]. ENVIRONMENTAL HEALTH PERSPECTIVES, 2020, 128 (02)
  • [3] Characteristics and source apportionment of VOCs measured in an industrial area of Nanjing, Yangtze River Delta, China
    An, Junlin
    Zhu, Bin
    Wang, Honglei
    Li, Yongyu
    Lin, Xu
    Yang, Hui
    [J]. ATMOSPHERIC ENVIRONMENT, 2014, 97 : 206 - 214
  • [4] Pollution profiles and health risk assessment of VOCs emitted during e-waste dismantling processes associated with different dismantling methods
    An, Taicheng
    Huang, Yong
    Li, Guiying
    He, Zhigui
    Chen, Jiangyao
    Zhang, Chaosheng
    [J]. ENVIRONMENT INTERNATIONAL, 2014, 73 : 186 - 194
  • [5] [Anonymous], 2017, The Global E -Waste Monitor 2017
  • [6] Ly BT, 2020, CHEMOSPHERE, V254, DOI 10.1016/j.chemosphere.2020.126749
  • [7] Atmospheric concentrations of SO2, NO2, ozone and VOCs in Duzce, Turkey using passive air samplers: Sources, spatial and seasonal variations and health risk estimation
    Bozkurt, Zehra
    Uzmez, Ozlem Ozden
    Dogeroglu, Tuncay
    Artun, Gulzade
    Gaga, Eftade O.
    [J]. ATMOSPHERIC POLLUTION RESEARCH, 2018, 9 (06) : 1146 - 1156
  • [8] Source identification and apportionment of volatile organic compounds in Houston, TX
    Buzcu, B
    Fraser, MP
    [J]. ATMOSPHERIC ENVIRONMENT, 2006, 40 (13) : 2385 - 2400
  • [9] VOCs elimination and health risk reduction in e-waste dismantling workshop using integrated techniques of electrostatic precipitation with advanced oxidation technologies
    Chen, Jiangyao
    Huang, Yong
    Li, Guiying
    An, Taicheng
    Hu, Yunkun
    Li, Yunlu
    [J]. JOURNAL OF HAZARDOUS MATERIALS, 2016, 302 : 395 - 403
  • [10] Relationship between environmental exposure to toluene, xylene and ethylbenzene and the expired breath concentrations for gasoline service workers
    Chen, ML
    Chen, SH
    Guo, BR
    Mao, IF
    [J]. JOURNAL OF ENVIRONMENTAL MONITORING, 2002, 4 (04): : 562 - 566