Volatile organic compounds in an e-waste dismantling region: From spatial-seasonal variation to human health impact

被引:45
作者
Chen, Daijin [1 ]
Liu, Ranran [1 ]
Lin, Qinhao [1 ,2 ]
Ma, Shengtao [1 ,2 ]
Li, Guiying [1 ,2 ]
Yu, Yingxin [1 ,2 ]
Zhang, Chaosheng [3 ,4 ]
An, Taicheng [1 ,2 ]
机构
[1] Guangdong Univ Technol, Inst Environm Hlth & Pollut Control, Guangdong Key Lab Environm Catalysis & Hlth Risk, Guangdong Hong Kong Macao Joint Lab Contaminants, Guangzhou 510006, Peoples R China
[2] Guangdong Univ Technol, Sch Environm Sci & Engn, Guangdong Technol Res Ctr Photocatalyt Technol In, Guangzhou Key Lab Environm Catalysis & Pollut Con, Guangzhou 510006, Peoples R China
[3] Natl Univ Ireland, GIS Ctr, Ryan Inst, Galway, Ireland
[4] Natl Univ Ireland, Sch Geog & Archaeol, Galway, Ireland
基金
中国国家自然科学基金;
关键词
Volatile organic compounds; E-waste dismantling region; Seasonal variation; Spatial distribution; Source apportionment; Health risk; AMBIENT MIXING RATIOS; YANGTZE-RIVER DELTA; SOURCE APPORTIONMENT; RISK-ASSESSMENT; POLLUTION PROFILES; ELECTRONIC WASTE; INDUSTRIAL-AREA; OZONE FORMATION; VOCS; EXPOSURE;
D O I
10.1016/j.chemosphere.2021.130022
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Y The dismantling of electrical and electronic waste (e-waste) can release various Volatile organic compounds (VOCs), impacting the surrounding ambient environment. We investigated the spatio-temporal characteristics and health risks of the ambient VOCs emitted in a typical e-waste dismantling region by conducting multi-site sampling campaigns in four seasons. The pollution of benzene, toluene, ethylbenzene, and xylenes (BTEX) in the e-waste dismantling park has relation to e-waste dismantling by seasonal trend analysis. The highest concentrations of most VOCs occurred in winter and autumn, while the lowest levels were observed in summer and spring. The spatial distribution map revealed the e-waste dismantling park to be a hotspot of BTEX, 1,2-dichloropropane (1,2-DCP), and 1,2-dichloroethane (1,2-DCA), while two major residential areas were also the hotspots of BTEX. The e-waste emission source contributed 20.14% to the total VOCs in the e-waste dismantling park, while it was absent in the major residential and rural areas. The cancer risk assessment showed that six VOCs exceeded 1.0 x 10(-6) in the e-waste dismantling park, while only three or four compounds exceeded this risk in other areas. The noncancer risks of all compounds were below the safety threshold. This study supplements the existing knowledge on VOC pollution from e-waste dismantling and expands the research scope of chemical pollution caused by e-waste. (C) 2021 Elsevier Ltd. All rights reserved.
引用
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页数:9
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