Structural Engineering of Covalent Organic Frameworks for Rechargeable Batteries

被引：84

作者：

Zhou, Limin ^{[1
]}

Jo, Seonyong ^{[1
]}

Park, Mihui ^{[2
]}

Fang, Liang ^{[2
]}

Zhang, Kai ^{[3
]}

Fan, Yanpeng ^{[3
]}

Hao, Zhimeng ^{[3
]}

Kang, Yong-Mook ^{[1
]}

机构：

[1] Korea Univ, Dept Mat Sci & Engn, 145 Anam Ro, Seoul 02841, South Korea

[2] Dongguk Univ Seoul, Dept Energy & Mat Engn, Seoul 100715, South Korea

[3] Nankai Univ, Coll Chem, Renewable Energy Convers & Storage Ctr, Key Lab Adv Energy Mat Chem,Minist Educ, Tianjin 300071, Peoples R China

来源：

ADVANCED ENERGY MATERIALS | 2021年 / 11卷 / 27期

基金：

新加坡国家研究基金会;

关键词：

covalent organic frameworks; ordered arrangements; porous materials; rechargeable batteries; structural engineering; CONJUGATED MICROPOROUS POLYMERS; ENERGY-STORAGE; CATHODE MATERIALS; CARBON NANOTUBES; LITHIUM STORAGE; ION BATTERIES; CYCLE LIFE; PERFORMANCE; NANOSHEETS; EFFICIENT;

D O I：

10.1002/aenm.202003054

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The structural designability of organic materials lays an optimal foundation for comprehensive energy-storage applications, owing to their selectivity of functional groups, diversity of linkage modes, and operability of synthesis conditions. Covalent organic frameworks (COFs), as a notable ordered porous framework structure, can provide a specific direction for ion diffusion as well as control the amount and location of redox sites, which are believed to be potential energy-storage or ion-transport carriers. In this study, a systematic overview of COFs for battery application is provided by conducting a comprehensive analysis and offering objective comments on the plasticity of the dominant structure and the improvement of the electrochemical properties. In addition, the existing problems and corresponding solutions of COFs for different devices are elaborated, and future research directions and application prospects of COFs are proposed. This review would provide theoretical guidance for alternative energy-storage materials and widen the applications of such promising materials for next-generation energy-storage devices.

引用

页数：34

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