On the use of double-skinned membranes to prevent chemical interaction between membranes and catalysts

被引：7

作者：

Arratibel, Alba ^{[1
]}

Tanaka, Alfredo Pacheco ^{[1
]}

van Sint Annaland, Martin ^{[2
]}

Gallucci, Fausto ^{[3
]}

机构：

[1] Tecnalia, Energy & Environm Div, Mikeletegi Pasealekua 2, San Sebastian 20009, Spain

[2] Eindhoven Univ Technol, Dept Chem Engn & Chem, Chem Proc Intensificat, Dolech 2,Rondom 70, NL-5612 AP Eindhoven, Netherlands

[3] Eindhoven Univ Technol, Dept Chem Engn & Chem, Sustainable Proc Engn, Inorgan Membranes & Membrane Reactors, Rondom 70, NL-5612 AP Eindhoven, Netherlands

来源：

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2021年 / 46卷 / 38期

关键词：

Pd-based membranes; Double-skin; Hydrogen separation; TiO2; catalyst; WATER-GAS-SHIFT; PT-RE/ZRO2; CATALYSTS; PALLADIUM MEMBRANE; MESOPOROUS TITANIA; PT-RE/TIO2; RUTILE; GOLD CATALYSTS; PD; INTERFACE; MECHANISM; SUPPORT;

D O I：

10.1016/j.ijhydene.2019.10.203

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

This communication summarizes the use of double-skinned membranes for hydrogen separation in presence of TiO2 based catalyst (PtReCe/TiO2). The use of this type of membrane avoids the direct contact between catalyst particles and surface of the Pd-based hydrogen selective layer due to the presence of a mesoporous YSZ/g-Al2O3 layer. The PdAg layer is protected by the mesoporous layer from direct contact with catalyst particles, avoiding erosion and possible chemical interactions. In comparison with a conventional PdAg membrane, the hydrogen flux of DS-membrane was observed not to be compromised during test carried out at 400 degrees C. (C) 2019 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

引用

页码：20240 / 20244

页数：5

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