Giant phonon softening in ferromagnetic LaMnO3+δ

被引:0
作者
Pashkevich, YG [1 ]
Gnezdilov, VP [1 ]
Lemmens, P [1 ]
Choi, KY [1 ]
Güntherodt, G [1 ]
Yeremenko, AV [1 ]
Barilo, SN [1 ]
Shiryaev, SV [1 ]
Soldatov, AG [1 ]
机构
[1] AA Galkin Donetsk Phystech NASU, UA-83114 Donetsk, Ukraine
来源
SPECTROSCOPY OF EMERGING MATERIALS | 2004年 / 165卷
关键词
manganites; Raman light scattering; orbital degrees of freedom;
D O I
暂无
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
High quality single crystals of LaMnO3+delta with delta = 0.071, 0.085, 0.092, 0.097, 0.125 that extend from antiferromagnetic insulating (delta = 0.071, T-N = 128 K) to ferromagnetic metallic state (delta = 0.125, T-C = 248 K) have been investigated by polarized Raman light scattering. A giant softening up to 30 cm(-1) of the 490- and 620-cm(-1) phonon modes has been observed below the Curie temperature. We interpret this phenomenon as a manifestation of an orbital fluctuating state which exists in a wide temperature range in ferromagnetic LaMnO3+delta.
引用
收藏
页码:185 / 194
页数:10
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