Preparation and characterization of F-modified C-TiO2 and its photocatalytic properties

被引:14
作者
Deng, Qin [1 ]
Liu, Yan [1 ]
Mu, Kangsheng [1 ]
Zeng, Yongmei [2 ]
Yang, Gang [1 ]
Shen, Fei [1 ]
Deng, Shihuai [1 ]
Zhang, Xiaohong [1 ]
Zhang, Yanzong [1 ]
机构
[1] Sichuan Agr Univ, Coll Resources & Environm, Country Sichuan Engn & Tech Ctr Rural Environm Pr, Chengdu 611130, Sichuan, Peoples R China
[2] Lib Sichuan Agr Univ, Dept Informat Integrat & Consultat, Chengdu 611130, Sichuan, Peoples R China
来源
PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE | 2015年 / 212卷 / 03期
关键词
nanocomposites; photocatalysis; TiO2; TIO2 NANOTUBE ARRAYS; N-DOPED TIO2; SOLVOTHERMAL SYNTHESIS; ANATASE TIO2; LIGHT; DEGRADATION; PERFORMANCE; CO; FACETS; NANOSTRUCTURES;
D O I
10.1002/pssa.201431805
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
F-modified C-doped TiO2 composites (CF-TiO2) were synthesized via a simple sol-gel method by using NaF as the fluorine source followed by heat treatment at 700 degrees C in nitrogen atmosphere. The as-prepared CF-TiO2 composites were characterized via transmission electron microscopy, Xray diffraction, N-2 sorption, X-ray photoelectron spectroscopy, UV-Vis diffuse reflectance spectroscopy, and photoluminescence. Carbon was doped into the anatase titania lattice, and the surface of C-doped TiO2 were modified by fluorine species. The CF-TiO2 composite showed excellent photocatalytic activity in degrading methylene blue under sunlight and simulated sunlight irradiation. (C) 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
引用
收藏
页码:691 / 697
页数:7
相关论文
共 32 条
[1]   Enhanced visible light-induced photoelectrocatalytic degradation of phenol by carbon nanotube-doped TiO2 electrodes [J].
Chen, Lung-Chuan ;
Ho, Yi-Ching ;
Guo, Wei-Sheng ;
Huang, Chao-Ming ;
Pan, Ting-Chung .
ELECTROCHIMICA ACTA, 2009, 54 (15) :3884-3891
[2]   Doping TiO2 with p-block elements: Effects on photocatalytic activity [J].
Dozzi, Maria Vittoria ;
Selli, Elena .
JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY C-PHOTOCHEMISTRY REVIEWS, 2013, 14 :13-28
[3]   Coincorporation of N and Ta into TiO2 Nanowires for Visible Light Driven Photoelectrochemical Water Oxidation [J].
Hoang, Son ;
Guo, Siwei ;
Mullins, C. Buddie .
JOURNAL OF PHYSICAL CHEMISTRY C, 2012, 116 (44) :23283-23290
[4]   Influence of crystal facets and F-modification on the photocatalytic performance of anatase TiO2 [J].
Li, Xi ;
Zhu, Jian ;
Li, Hexing .
CATALYSIS COMMUNICATIONS, 2012, 24 :20-24
[5]   Enhanced photocatalytic activity of fluorine doped TiO2 by loaded with Ag for degradation of organic pollutants [J].
Lin, Xiaoxia ;
Rong, Fei ;
Fu, Degang ;
Yuan, Chunwei .
POWDER TECHNOLOGY, 2012, 219 :173-178
[6]   New insights into the origin of visible light photocatalytic activity of nitrogen-doped and oxygen-deficient anatase TiO2 [J].
Lin, ZS ;
Orlov, A ;
Lambert, RM ;
Payne, MC .
JOURNAL OF PHYSICAL CHEMISTRY B, 2005, 109 (44) :20948-20952
[7]   Visible-light photocatalytic degradation of methyl orange by CdS-TiO2-Au composites synthesized via microwave-assisted reaction [J].
Lv, Tian ;
Pan, Likun ;
Liu, Xinjuan ;
Sun, Zhuo .
ELECTROCHIMICA ACTA, 2012, 83 :216-220
[8]   TiO2 wrapped graphene as a high performance photocatalyst for acid orange 7 dye degradation under solar/UV light irradiations [J].
Muthirulan, P. ;
Devi, C. Nirmala ;
Sundaram, M. Meenakshi .
CERAMICS INTERNATIONAL, 2014, 40 (04) :5945-5957
[9]   A review on the visible light active titanium dioxide photocatalysts for environmental applications [J].
Pelaez, Miguel ;
Nolan, Nicholas T. ;
Pillai, Suresh C. ;
Seery, Michael K. ;
Falaras, Polycarpos ;
Kontos, Athanassios G. ;
Dunlop, Patrick S. M. ;
Hamilton, Jeremy W. J. ;
Byrne, J. Anthony ;
O'Shea, Kevin ;
Entezari, Mohammad H. ;
Dionysiou, Dionysios D. .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2012, 125 :331-349
[10]   Origin of the Visible Light Absorption of Boron/Nitrogen Co-doped Anatase TiO2 [J].
Sun, Chenghua ;
Searles, Debra J. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2013, 117 (50) :26454-26459