Pure organic quinacridone dyes as dual sensitizers in tandem photoelectrochemical cells for unassisted total water splitting

被引:12
|
作者
Shen, Luze [1 ]
Zhang, Shicong [1 ]
Ding, Haoran [1 ]
Niu, Fushuang [2 ]
Chu, Yanmeng [3 ]
Wu, Wenjun [1 ]
Hu, Yue [3 ]
Hu, Ke [2 ]
Hua, Jianli [1 ]
机构
[1] East China Univ Sci & Technol, Sch Chem & Mol Engn, Inst Fine Chem, Key Lab Adv Mat, 130 Meilong Rd, Shanghai 200237, Peoples R China
[2] Fudan Univ, Dept Chem, 220 Handan Rd, Shanghai 200433, Peoples R China
[3] Huazhong Univ Sci & Technol, Wuhan Natl Lab Optoelect, Michael Gratzel Ctr Mesoscop Solar Cells, 1056 Luoyu Rd, Wuhan 430074, Hubei, Peoples R China
基金
中国国家自然科学基金;
关键词
DRIVEN HYDROGEN-PRODUCTION; ELECTRON-TRANSFER; SOLAR-CELLS; OXIDATION; CATALYST; PHOTOCATHODES; CHROMOPHORE; EXCHANGE; DESIGN;
D O I
10.1039/d1cc01570b
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Pure organic dye QAP-C8 based on quinacridone (QA) with octyl side chains as the donor and pyridine dicarboxylic acid (PDA) as the acceptor was first used in both the photoanode and the photocathode of photoelectrochemical cells. A tandem device with QAP-C8 as the photosensitizer realized overall water splitting and showed a STH of 0.11% under neutral pH conditions without an external bias.
引用
收藏
页码:5634 / 5637
页数:4
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