High-sensitivity electron paramagnetic resonance of Mn12-acetate

被引：242

作者：

Hill, S ^{[1
]}

Perenboom, JAAJ

Dalal, NS

Hathaway, T

Stalcup, T

Brooks, JS

机构：

[1] Montana State Univ, Dept Phys, Bozeman, MT 59717 USA

[2] Catholic Univ Nijmegen, Mat Res Inst, NL-6525 ED Nijmegen, Netherlands

[3] Catholic Univ Nijmegen, High Field Magnet Lab, NL-6525 ED Nijmegen, Netherlands

[4] Florida State Univ, Dept Chem, Tallahassee, FL 32310 USA

[5] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA

来源：

PHYSICAL REVIEW LETTERS | 1998年 / 80卷 / 11期

关键词：

D O I：

10.1103/PhysRevLett.80.2453

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

The energy diagram of Mn-12-acetate is probed close to the top of the anisotropy barrier using a novel, high-sensitivity, electron paramagnetic resonance technique. Multiple resonances, and their temperature dependence, are observed from 35 to 115 GHz, for a single high-quality crystal. The data are sufficiently detailed to make extremely accurate comparisons with predictions based on a spin S = 10 Hamiltonian. Although overall agreement is good, we find evidence for possible inadequacies of this model.

引用

页码：2453 / 2456

页数：4

共 15 条

[1] High-frequency EPR spectra of a molecular nanomagnet: Understanding quantum tunneling of the magnetization [J].