Geological interactions and radio-chemical risks of primordial radionuclides 40K, 226Ra, and 232Th in soil and groundwater from potential radioactive waste disposal site in Ghana

被引:18
作者
Akortia, Eric [1 ]
Glover, Eric T. [1 ,2 ]
Nyarku, Mawutorli [2 ]
Dawood, Abdallah M. A. [1 ]
Essel, Paul [1 ]
Sarfo, Evelyn Ofosu [1 ]
Ameho, Evans M. [1 ]
Aberikae, Emmanuel A. [1 ]
Gbeddy, Gustav [1 ]
机构
[1] Ghana Atom Energy Commiss, Radiat Protect Inst, Radioact Waste Management Ctr, POB LG 80, Legon, Accra, Ghana
[2] Univ Ghana, Sch Nucl & Allied Sci, Coll Sci, Legon, Accra, Ghana
关键词
Natural radioactivity; Radio-chemical risk; Multi-criteria decision making; Gamma spectrometry; Annual gonadal equivalent dose; Annual effective ingestion dose; DRINKING-WATER; NATURAL RADIOACTIVITY; SPATIAL-DISTRIBUTION; COASTAL SEDIMENTS; EASTERN DESERT; HEALTH-RISK; URANIUM; HAZARDS; TAMILNADU; EXPOSURE;
D O I
10.1007/s10967-021-07675-2
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
This study assessed the influence of geological depth and formation on activity concentrations of Th-232, Ra-226 and K-40 in soil and groundwater, and radio-chemical health risks. Preference ranking organisation method for enrichment evaluation and geometrical analysis for interactive aid indicated significant correlation between Th-232 and K-40, thus indicating potential similar primordial origin. Deepest depth rocks at 145 m and 148 m constituted of dark coloured silicified schist exhibited minimal activity with potential hydro-geological interactions with groundwater. Age-dependent annual effective ingestion dose for Ra-226 and Th-232 are higher than the UNSCEAR reference dose, thus the groundwater is unsuitable for long-term consumption.
引用
收藏
页码:577 / 589
页数:13
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