Aerosol optical properties under different pollution levels in the Pearl River Delta (PRD) region of China

被引:30
|
作者
Kong, Liuwei [1 ]
Hu, Min [2 ]
Tan, Qinwen [3 ]
Feng, Miao [3 ]
Qu, Yu [4 ]
An, Junling [4 ]
Zhang, Yuanhang [2 ]
Liu, Xingang [1 ]
Cheng, Nianliang [5 ]
机构
[1] Beijing Normal Univ, Sch Environm, State Key Lab Water Environm Simulat, Beijing 100875, Peoples R China
[2] Peking Univ, Coll Environm Sci & Engn, Beijing 100871, Peoples R China
[3] Chengdu Acad Environm Sci, Chengdu 610072, Sichuan, Peoples R China
[4] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China
[5] Beijing Municipal Environm Monitoring Ctr, Beijing 100048, Peoples R China
来源
JOURNAL OF ENVIRONMENTAL SCIENCES | 2020年 / 87卷
基金
中国国家自然科学基金;
关键词
Particulate aerosol; Hygroscopic growth; Optical properties; PRD; MEGA-CITY GUANGZHOU; HYGROSCOPIC GROWTH; CHEMICAL-COMPOSITION; FORMATION MECHANISM; SCATTERING COEFFICIENT; SOURCE APPORTIONMENT; RELATIVE-HUMIDITY; HAZE FORMATION; RURAL AREA; PM2.5;
D O I
10.1016/j.jes.2019.02.019
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
To clarify the aerosol hygroscopic growth and optical properties of the Pearl River Delta (PRD) region, integrated observations were conducted in Heshan City of Guangdong Province from October 19 to November 17, 2014. The concentrations and chemical compositions of PM2.5, aerosol optical properties and meteorological parameters were measured. The mean value of PM2.5 increased from less than 35 (excellent) to 35-75 mu g/m(3) (good) and then to greater than 75 mu g/m(3) (pollution), corresponding to mean PM2.5 values of 24.9, 51.2, and 93.3 mu g/m(3), respectively. The aerosol scattering hygroscopic growth factor (f(RH = 80%)) values were 2.0, 2.12, and 2.18 for the excellent, good, and pollution levels, respectively. The atmospheric extinction coefficient (sigma(ext)) and the absorption coefficient of aerosols (sigma(ap)) increased, and the single scattering albedo (SSA) decreased from the excellent to the pollution levels. For different air mass sources, under excellent and good levels, the land air mass from northern Heshan had lower f(RH) and sigma(sp) values. In addition, the mixed aerosol from the sea and coastal cities had lower f(RH) and showed that the local sources of coastal cities have higher scattering characteristics in pollution periods. (c) 2019 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
引用
收藏
页码:49 / 59
页数:11
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