Amine-functionalized natural zeolites prepared through plasma polymerization for enhanced carbon dioxide adsorption

被引：13

作者：

Wahono, Satriyo K. ^{[1
,2
]}

Dwiatmoko, Adid A. ^{[3
]}

Cavallaro, Alex ^{[1
]}

Indirathankam, Sathish C. ^{[4
]}

Addai-Mensah, Jonas ^{[1
]}

Skinner, William ^{[1
]}

Vinu, Ajayan ^{[1
,4
]}

Vasilev, Krasimir ^{[1
,5
]}

机构：

[1] Univ South Australia, Future Ind Inst, Mawson Lakes, SA, Australia

[2] Indonesian Inst Sci, Res Div Nat Prod Technol, Yogyakarta, Indonesia

[3] PUSPIPTEK Serpong, Indonesian Inst Sci, Res Ctr Chem, Tangerang Selatan, Indonesia

[4] Univ Newcastle, Fac Engn & Built Environm, Global Innovat Ctr Adv Nanomat, Callaghan, NSW, Australia

[5] Univ South Australia, Acad Unit STEM, Adelaide, SA, Australia

来源：

PLASMA PROCESSES AND POLYMERS | 2021年 / 18卷 / 08期

关键词：

allylamine; CO2 adsorption capacity; natural mordenite– clinoptilolite zeolite; plasma deposition; plasma polymerization; CO2; CAPTURE; SURFACES; TECHNOLOGY; GENERATION; SORBENTS; REMOVAL;

D O I：

10.1002/ppap.202100028

中图分类号：

O59 [应用物理学];

学科分类号：

摘要：

Solution-based amine absorption technologies have been widely applied for CO2 capture, but they have several drawbacks. This paper reports on the synthesis of the first solid-state amine adsorbent prepared through a simple plasma polymerization and deposition on physicochemically modified natural mordenite-clinoptilolite zeolite. The plasma deposition of amine polymer under certain conditions resulted in a significant increase in surface area-weighted CO2 adsorption capacity as the natural zeolite. The strength of the interaction between CO2 and the adsorbent was weaker for the plasma polymer-modified zeolite than without the plasma coating, which may facilitate regeneration. Both indications make the amine plasma polymer-based zeolite adsorbent a good candidate for CO2 adsorption and separation.

引用

页数：11

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