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Effectively promoted catalytic activity by adjusting calcination temperature of Ce-Fe-Ox catalyst for NH3-SCR
被引:13
作者:

Song, Zhongxian
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Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China

Xing, Yun
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Shenyang Univ Chem Technol, Coll Environm & Safety Engn, Shenyang 110142, Liaoning, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China

Zhang, Tingji
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Shenyang Univ Chem Technol, Coll Environm & Safety Engn, Shenyang 110142, Liaoning, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China

Zhao, Jinggang
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Shenyang Univ Chem Technol, Coll Environm & Safety Engn, Shenyang 110142, Liaoning, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China

Wang, Junkai
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Shenyang Univ Chem Technol, Coll Environm & Safety Engn, Shenyang 110142, Liaoning, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China

Mao, Yanli
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Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China

Zhao, Baolin
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Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China

Zhang, Xuejun
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机构:
Shenyang Univ Chem Technol, Coll Environm & Safety Engn, Shenyang 110142, Liaoning, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China

Zhao, Min
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Shenyang Univ Chem Technol, Coll Environm & Safety Engn, Shenyang 110142, Liaoning, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China

Ma, Ziang
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h-index: 0
机构:
Shenyang Univ Chem Technol, Coll Environm & Safety Engn, Shenyang 110142, Liaoning, Peoples R China Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China
机构:
[1] Henan Univ Urban Construct, Fac Environm & Municipal Engn, Henan Key Lab Water Pollut Control & Rehabil Tech, Pingdingshan 467000, Peoples R China
[2] Shenyang Univ Chem Technol, Coll Environm & Safety Engn, Shenyang 110142, Liaoning, Peoples R China
基金:
中国国家自然科学基金;
关键词:
calcination temperatures;
selectivity catalytic reduction;
sulfate species;
surface acidity;
NO REDUCTION;
ENHANCED PERFORMANCE;
MIXED OXIDES;
NH3;
CERIA;
SCR;
AMMONIA;
SO2;
COMBUSTION;
RESISTANCE;
D O I:
10.1002/aoc.5446
中图分类号:
O69 [应用化学];
学科分类号:
081704 ;
摘要:
A series of Ce-Fe-O-x catalysts prepared by the different calcination temperatures (marked as CF-X, where X represented calcination temperature) were used to the selectivity catalytic reduction of NOx by NH3. The results explained the relationship between calcination temperature and the sulfate species over Ce-Fe-O-x, and then investigated the surface acidity and catalytic performance. The large amounts of sulfate species were formed over CF-450 and CF-550 while it was decomposed with further the increasing of calcination temperature, which resulted in the loss of surface acidity, causing a decrease in the catalytic activity over Ce-Fe-O-x. Thereby, the CF-450 catalyst showed the best catalytic activity and over 90% NOx conversion was obtained at 244-450 degrees C. Besides, the favored pore structure, more Fe3+ active species, higher Ce3+ concentration and the abundance of chemical adsorbed oxygen species, as well as the surface acid sites, would together contribute to the excellent catalytic activity of CF-450 catalyst.
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页数:9
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