Photocatalytic performance of TiO2-zeolite templated carbon composites in organic contaminant degradation

被引:24
作者
Donphai, Waleeporn [1 ,2 ]
Kamegawa, Takashi [1 ,3 ]
Chareonpanich, Metta [2 ]
Nueangnoraj, Khanin [4 ]
Nishihara, Hirotomo [4 ]
Kyotani, Takashi [4 ]
Yamashit, Hiromi [1 ,5 ]
机构
[1] Osaka Univ, Grad Sch Engn, Div Mat & Mfg Sci, Suita, Osaka 5650871, Japan
[2] Kasetsart Univ, Fac Engn, Dept Chem Engn, Bangkok 10900, Thailand
[3] Osaka Prefecture Univ, Nanosci & Nanotechnol Res Ctr, Naka Ku, Sakai, Osaka 5998570, Japan
[4] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
[5] Kyoto Univ, ESICB, Katsura, Kyoto 6158520, Japan
关键词
AREA MICROPOROUS CARBON; MESOPOROUS SILICA; TIO2; PHOTODEGRADATION; NANOTUBES; BENZENE; STORAGE;
D O I
10.1039/c4cp03897e
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
TiO2 composites with zeolite templated carbon (TiO2-ZTC) and activated carbon (TiO2-AC) were prepared and used as the photocatalysts for comparative studies with pure TiO2. TiO2-ZTC exhibited the highest rate of methylene blue degradation with a rate approximately 4 and 400 times higher than those of TiO2-AC and pure TiO2, respectively. Moreover, the highest catalytic performance of TiO2-ZTC in gas-phase degradation of acetone was approximately 1.1 and 12.9 times higher than TiO2-AC and pure TiO2, respectively. These outstanding performances could be attributed to high surface area, pore volume, and hydrophobic surface properties, leading to improvement in the adsorption properties of organic molecules.
引用
收藏
页码:25004 / 25007
页数:4
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