Production of gas hydrate in a semi-batch spray reactor process as a means for separation of carbon dioxide from methane

被引:54
作者
Partoon, Behzad [1 ]
Sabil, Khalik M. [2 ]
Lau, Kok Keong [1 ]
Lal, Bhajan [1 ]
Nasrifar, Khashayar [3 ]
机构
[1] Univ Teknol PETRONAS, Inst Contaminat Management, Res Ctr CO2, Bandar Seri Iskandar 32610, Perak Darul Rid, Malaysia
[2] Heriot Watt Univ Malaysia, Sch Energy Geosci Infrastruct & Soc, Inst Petr Engn, 1 Jalan Venna P5-2,Precinct 5, Putrajaya 62200, Federal Territo, Malaysia
[3] Shiraz Univ Technol, Chem Petr & Gas Engn Dept, Modares Blv 71557-13876, Shiraz, Fars, Iran
关键词
Process; Gas hydrate; Spray reactor; Carbon dioxide; Separation; PRE-COMBUSTION CAPTURE; CO2; CAPTURE; FLUE-GAS; MIXTURES; RECOVERY; ADSORPTION;
D O I
10.1016/j.cherd.2018.08.024
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
The formation of gas hydrate shows good potential to work as a separation medium for gas mixtures. However, to put it in practice, the impact of process parameters, such as flow rates, operational temperature and pressure are required to be adequately investigated. In this work, a new gas hydrate reactor is introduced for fast production of gas hydrate. The reactor is used for separation of carbon dioxide from methane in a series of semi-batch experiments. Results indicated that fast hydrate production is achievable. In addition, carbon dioxide is effectively separated from methane by producing gas hydrate from a gas mixture containing more than 60% carbon dioxide. (C) 2018 Institution of Chemical Engineers. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:168 / 175
页数:8
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