Nitrogen-Doped Graphene as Efficient Metal-Free Electrocatalyst for Oxygen Reduction in Fuel Cells

被引:3573
作者
Qu, Liangti [2 ]
Liu, Yong [1 ]
Baek, Jong-Beom [3 ]
Dai, Liming [4 ]
机构
[1] Wenzhou Med Coll, Sch Ophthalmol & Optometry, Biomed Engn Acad, Wenzhou 325027, Zhejiang, Peoples R China
[2] Beijing Inst Technol, Sch Sci, Dept Chem, Beijing 100081, Peoples R China
[3] UNIST, Sch Energy Engn, Ulsan 681800, South Korea
[4] Case Western Reserve Univ, Dept Chem Engn, Cleveland, OH 44106 USA
基金
新加坡国家研究基金会;
关键词
graphene; N-doping; oxygen reduction; fuel cell; CHEMICAL-VAPOR-DEPOSITION; WALL CARBON NANOTUBES; FILMS; SHEETS; NANOCOMPOSITE; ELECTRODES; GRAPHITE; CRYSTALS; SINGLE;
D O I
10.1021/nn901850u
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Nitrogen-doped graphene (N-graphene) was synthesized by chemical vapor deposition of methane in the presence of ammonia. The resultant N-graphene was demonstrated to act as a metal-free electrode with a much better electrocatalytic activity, long-term operation stability, and tolerance to crossover effect than platinum for oxygen reduction via a four-electron pathway in alkaline fuel cells. To the best of our knowledge, this is the first report on the use of graphene and its derivatives as metal-free catalysts for oxygen reduction. The important role of N-doping to oxygen reduction reaction (ORR) can be applied to various carbon materials for the development of other metal-free efficient ORR catalysts for fuel cell applications, even new catalytic materials for applications beyond fuel cells.
引用
收藏
页码:1321 / 1326
页数:6
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