Degradation and regeneration of copper-iron spinel and zeolite composite catalysts in steam reforming of dimethyl ether
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作者:
Shimoda, N.
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Shimoda, N.
[1
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Faungnawakij, K.
[1
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Kikuchi, R.
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Kikuchi, R.
[1
]
Eguchi, K.
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Eguchi, K.
[1
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机构:
[1] Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
The degradation and regeneration behaviors of some composite catalysts of ZSM-5 zeolite and Cu-Fe spinel in steam reforming of dimethyl ether (DME) were systematically studied in various conditions. The degradation of the catalyst could be inhibited by increasing the steam-to-DME ratio and/or lowering the gas hourly space velocity and the reforming temperature. A higher mixing ratio of Cu-Fe spinel to ZSM-5 could also prolong the life of the composite catalysts. The catalyst deactivation was attributable mainly to the carbon deposition in the reaction temperature range of 250-310 degrees C. The regeneration treatment in air at 500-700 degrees C could not only recover the catalytic performance of the degraded catalysts as compared with the fresh catalyst, but could also improve it. We confirmed that the promoting effect of the heat treatment in air was due to the high redispersion of metallic Cu via the re-construction of Cu-Fe spinel as well to as the removal of carbon deposit by burning; the acid property changes over zeolite catalyst were suggested to contribute to the improvement as well. (C) 2010 Elsevier B.V. All rights reserved.
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Eguchi, K.
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Shimoda, N.
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Shimoda, N.
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Faungnawakij, K.
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Matsui, T.
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Matsui, T.
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Kikuchi, R.
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Kikuchi, R.
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Kawashima, S.
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Japan Sci & Technol Agcy, Nishikyo Ku, Kyoto 6158245, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
机构:
Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Japan Sci & Technol Agcy, Nishikyo Ku, Kyoto 6158245, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Faungnawakij, Kajomsak
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Fukunaga, Tetsuya
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Idemitsu Kosan Co Ltd, Cent Res Labs, Chiba 2990293, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Fukunaga, Tetsuya
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Kikuchi, Ryuji
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Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Kikuchi, Ryuji
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Eguchi, Koichi
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Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
机构:Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Tanaka, Yohei
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Shimoda, Naohiro
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机构:Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Shimoda, Naohiro
;
Fukunaga, Tetsuya
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机构:Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Fukunaga, Tetsuya
;
Kikuchi, Ryuji
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机构:Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Kikuchi, Ryuji
;
Eguchi, Koichi
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Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
机构:
Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Kikuchi, Ryuji
;
Shimoda, Naohiro
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Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Shimoda, Naohiro
;
Fukunaga, Tetsuya
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h-index: 0
机构:
Idemitsu Kosan Co Ltd, Cent Res Labs, Chiba 2990293, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Fukunaga, Tetsuya
;
Eguchi, Koichi
论文数: 0引用数: 0
h-index: 0
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Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
机构:
Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Eguchi, K.
;
Shimoda, N.
论文数: 0引用数: 0
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Shimoda, N.
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Faungnawakij, K.
;
Matsui, T.
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Matsui, T.
;
Kikuchi, R.
论文数: 0引用数: 0
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Kyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
Kikuchi, R.
;
Kawashima, S.
论文数: 0引用数: 0
h-index: 0
机构:
Japan Sci & Technol Agcy, Nishikyo Ku, Kyoto 6158245, JapanKyoto Univ, Dept Energy & Hydrocarbon Chem, Grad Sch Engn, Nishikyo Ku, Kyoto 6158510, Japan
机构:
Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Japan Sci & Technol Agcy, Nishikyo Ku, Kyoto 6158245, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Faungnawakij, Kajomsak
;
Fukunaga, Tetsuya
论文数: 0引用数: 0
h-index: 0
机构:
Idemitsu Kosan Co Ltd, Cent Res Labs, Chiba 2990293, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Fukunaga, Tetsuya
;
Kikuchi, Ryuji
论文数: 0引用数: 0
h-index: 0
机构:
Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Kikuchi, Ryuji
;
Eguchi, Koichi
论文数: 0引用数: 0
h-index: 0
机构:
Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
机构:Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Tanaka, Yohei
;
Shimoda, Naohiro
论文数: 0引用数: 0
h-index: 0
机构:Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Shimoda, Naohiro
;
Fukunaga, Tetsuya
论文数: 0引用数: 0
h-index: 0
机构:Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Fukunaga, Tetsuya
;
Kikuchi, Ryuji
论文数: 0引用数: 0
h-index: 0
机构:Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Kikuchi, Ryuji
;
Eguchi, Koichi
论文数: 0引用数: 0
h-index: 0
机构:
Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
机构:
Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Kikuchi, Ryuji
;
Shimoda, Naohiro
论文数: 0引用数: 0
h-index: 0
机构:
Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Shimoda, Naohiro
;
Fukunaga, Tetsuya
论文数: 0引用数: 0
h-index: 0
机构:
Idemitsu Kosan Co Ltd, Cent Res Labs, Chiba 2990293, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan
Fukunaga, Tetsuya
;
Eguchi, Koichi
论文数: 0引用数: 0
h-index: 0
机构:
Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, JapanKyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan