What have we learnt about heavy carbenes through laser flash photolysis studies?

被引:61
作者
Becerra, Rosa
Walsh, Robin
机构
[1] Univ Reading, Sch Chem, Reading RG6 6AD, Berks, England
[2] CSIC, Inst Quim Fis Rocasolano, E-28006 Madrid, Spain
关键词
D O I
10.1039/b617844h
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Time resolved gas-phase kinetic studies have contributed a great deal of fundamental information about the reactions and reactivity of heavy carbenes (silylenes, germylenes and stannylenes) during the past two decades. In this article we trace the development of our understanding through the mechanistic themes of intermediate complexes, third body assisted associations, catalysed reactions, non-observed reactions and substituent effects. Ab initio (quantum chemical) calculations have substantially assisted mechanistic interpretation and are discussed where appropriate. Trends in reactivity are identified and some signposts to future studies are indicated. This review, although detailed, is not comprehensive.
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收藏
页码:2817 / 2835
页数:19
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