Cold neutron study on the diffuse scattering and phonon excitations in the relaxor Pb(Mg1/3Nb2/3)O3 -: art. no. 184105

被引:69
作者
Hiraka, H [1 ]
Lee, SH
Gehring, PM
Xu, GY
Shirane, G
机构
[1] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA
[2] Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, Japan
[3] Natl Inst Stand & Technol, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevB.70.184105
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Cold neutron scattering experiments have been performed to explore the energy, temperature, and wave-vector dependence of the diffuse scattering and the transverse acoustic (TA) phonons in the relaxor Pb(Mg1/3Nb2/3)O-3. We have observed a weak diffuse scattering cross section above the Burns temperature T(d)similar to600 K. This cross section, which is most likely caused by chemical short-range order, persists down to 100 K, and coexists with the much stronger diffuse scattering that is attributed to the polar nanoregions. A systematic study of the TA phonon around (1, 1, 0) has also been carried out. The phonon is well defined for small wave-vectors q, but broadens markedly around q=(0.1,-0.1,0).
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页码:1 / 7
页数:7
相关论文
共 25 条
[1]   GLASSY POLARIZATION BEHAVIOR IN FERROELECTRIC COMPOUNDS PB(MG1/3NB2/3)O3 AND PB(ZN1/3NB2/3)O3 [J].
BURNS, G ;
DACOL, FH .
SOLID STATE COMMUNICATIONS, 1983, 48 (10) :853-856
[2]   Why Pb(B1/3B′2/3)O3 perovskites disorder more easily than Ba(B1/3B′2/3)O3 perovskites and the thermodynamics of 1:1-type short-range order in PMN [J].
Burton, BP .
JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS, 2000, 61 (02) :327-333
[3]   Why Pb(B,B′)O3 perovskites disorder at lower temperatures than Ba(B,B′)O3 perovskites [J].
Burton, BP ;
Cockayne, E .
PHYSICAL REVIEW B, 1999, 60 (18) :R12542-R12545
[4]   Pressure-induced suppression of the diffuse scattering in the model relaxor ferroelectric PbMg1/3Nb2/3O3 -: art. no. 257601 [J].
Chaabane, B ;
Kreisel, J ;
Dkhil, B ;
Bouvier, P ;
Mezouar, M .
PHYSICAL REVIEW LETTERS, 2003, 90 (25) :4
[5]   Soft mode dynamics above and below the burns temperature in the relaxor Pb(Mg1/3Nb2/3)O3 -: art. no. 277601 [J].
Gehring, PM ;
Wakimoto, S ;
Ye, ZG ;
Shirane, G .
PHYSICAL REVIEW LETTERS, 2001, 87 (27) :277601-277601
[6]   Disorder and relaxation mode in the lattice dynamics of the PbMg1/3Nb2/3O3 relaxor ferroelectric -: art. no. 092105 [J].
Gvasaliya, SN ;
Lushnikov, SG ;
Roessli, B .
PHYSICAL REVIEW B, 2004, 69 (09)
[7]   On the existence of the relaxation mode in relaxor ferroelectrics [J].
Gvasaliya, SN ;
Lushnikov, SG ;
Roessli, B .
CRYSTALLOGRAPHY REPORTS, 2004, 49 (01) :108-113
[8]   Neutron diffuse scattering from polar nanoregions in the relaxor Pb(Mg1/3Nb2/3)O3 -: art. no. 104105 [J].
Hirota, K ;
Ye, ZG ;
Wakimoto, S ;
Gehring, PM ;
Shirane, G .
PHYSICAL REVIEW B, 2002, 65 (10) :1-7
[9]   Origin of the "Waterfall" effect in phonon dispersion of relaxor perovskites [J].
Hlinka, J ;
Kamba, S ;
Petzelt, J ;
Kulda, J ;
Randall, CA ;
Zhang, SJ .
PHYSICAL REVIEW LETTERS, 2003, 91 (10)
[10]   Diffuse scattering in Pb(Zn1/3Nb2/3)O3 with 8% PbTiO3 by quasi-elastic neutron scattering [J].
Hlinka, J ;
Kamba, S ;
Petzelt, J ;
Kulda, J ;
Randall, CA ;
Zhang, SJ .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2003, 15 (24) :4249-4257