Strong exciton-photon coupling and exciton hybridization in a thermally evaporated polycrystalline film of an organic small molecule

被引：138

作者：

Holmes, RJ ^{[1
]}

Forrest, SR ^{[1
]}

机构：

[1] Princeton Univ, Dept Elect Engn, Princeton Inst Sci & Technol Mat, Princeton, NJ 08544 USA

来源：

PHYSICAL REVIEW LETTERS | 2004年 / 93卷 / 18期

关键词：

D O I：

10.1103/PhysRevLett.93.186404

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We demonstrate strong exciton-photon coupling in an optical microcavity containing a thermally evaporated polycrystalline organic thin film. Microcavity polaritons result from coupling between the 0-0 excitonic transition of 3,4,7,8 napthalenetetracarboxylic dianhydride and a cavity photon. For thicker films, the 0-1 transition also couples to the cavity mode, as vibronic relaxation is overcome by the short Rabi period for strong coupling. To our knowledge, this is the first report of strong coupling between a cavity photon and multiple vibronic transitions in a single material, made possible by the pronounced vibronic absorption features characteristic of crystalline organic materials.

引用

页码：186404 / 1

页数：4

共 50 条

[31] Strong exciton-photon coupling in anthradithiophene microcavities: from isolated molecules to aggregates [J].

Van Schenck, J. D. B. ;

Tanyi, E. K. ;

Cheng, L. -J. ;

Anthony, J. ;

Ostroverkhova, O. .

MRS COMMUNICATIONS, 2019, 9 (03) :956-963

[32] Strong exciton–photon coupling in an organic semiconductor microcavity [J].

D. G. Lidzey ;

D. D. C. Bradley ;

M. S. Skolnick ;

T. Virgili ;

S. Walker ;

D. M. Whittaker .

Nature, 1998, 395 :53-55

[33] Observation of strong exciton-photon coupling in semiconductor microcavities containing organic dyes and J-aggregates [J].

Lidzey, D.G. ;

Virgili, T. ;

Bradley, D.D.C. ;

Skolnick, M.S. ;

Walker, S. ;

Whittaker, D.M. .

Optical Materials, 1999, 12 (02) :243-247

[34] Observation of strong exciton-photon coupling in semiconductor microcavities containing organic dyes and J-aggregates [J].

Lidzey, DG ;

Virgili, T ;

Bradley, DDC ;

Skolnick, MS ;

Walker, S ;

Whittaker, DM .

OPTICAL MATERIALS, 1999, 12 (2-3) :243-247

[35] Surface Plasmon Enhanced Strong Exciton-Photon Coupling in Hybrid Inorganic-Organic Perovskite Nanowires [J].

Shang, Qiuyu ;

Zhang, Shuai ;

Liu, Zhen ;

Chen, Jie ;

Yang, Pengfei ;

Li, Chun ;

Li, Wei ;

Zhang, Yanfeng ;

Xiong, Qihua ;

Liu, Xinfeng ;

Zhang, Qing .

NANO LETTERS, 2018, 18 (06) :3335-3343

[36] ON EXCITON-PHOTON COUPLING AND RETARDED INTERACTIONS IN MOLECULAR CRYSTALS [J].

PHILPOTT, MR .

JOURNAL OF PHYSICS PART C SOLID STATE PHYSICS, 1968, 1 (01) :42-&

[37] Ultrastrong Exciton-Photon Coupling in Broadband Solar Absorbers [J].

Bujalance, Clara ;

Esteso, Victoria ;

Calio, Laura ;

Lavarda, Giulia ;

Torres, Tomas ;

Feist, Johannes ;

Jose Garcia-Vidal, Francisco ;

Bottari, Giovanni ;

Miguez, Hernan .

JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2021, 12 (43) :10706-10712

[38] Polariton solitons due to saturation of the exciton-photon coupling [J].

Egorov, O. A. ;

Skryabin, D. V. ;

Lederer, F. .

PHYSICAL REVIEW B, 2010, 82 (16)

[39] Strong Exciton-Photon Coupling in Layered Perovskites Embedded Low-Q Microcavity [J].

Pradeesh, K. ;

Prakash, G. Vijaya .

INEC: 2010 3RD INTERNATIONAL NANOELECTRONICS CONFERENCE, VOLS 1 AND 2, 2010, :285-286

[40] Plasmonic effects on strong exciton-photon coupling in metal-insulator-metal microcavities [J].

Hayashi, Shinji ;

Ishigaki, Yuta ;

Fujii, Minoru .

PHYSICAL REVIEW B, 2012, 86 (04)

← 1 2 3 4 5 →