Quantum fluctuations and the magnetic ground state of Ce3Pd20Si6

被引：32

作者：

Deen, P. P. ^{[1
]}

Strydom, A. M. ^{[2
]}

Paschen, S. ^{[3
]}

Adroja, D. T. ^{[4
]}

Kockelmann, W. ^{[4
]}

Rols, S. ^{[1
]}

机构：

[1] Inst Laue Langevin, F-38042 Grenoble, France

[2] Univ Johannesburg, Phys Dept APK, ZA-2006 Aukland Pk, South Africa

[3] TU Wien, Inst Festkorperphys, A-1040 Vienna, Austria

[4] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England

来源：

PHYSICAL REVIEW B | 2010年 / 81卷 / 06期

基金：

奥地利科学基金会; 欧洲研究理事会;

关键词：

CRYSTAL-FIELD EXCITATIONS; R3PD20GE6; R; CRITICALITY; TRANSPORT; PR; CE;

D O I：

10.1103/PhysRevB.81.064427

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

The temperature and magnetic field dependence of neutron-scattering studies on the heavy fermion compound Ce3Pd20Si6 are reported. Inelastic neutron scattering reveals two crystal-field excitations corresponding to the environments of the two distinct rare-earth locations within this cubic compound. Surprisingly, the ground states of the two individual Ce sites are inequivalent with the 4a site having a Gamma(7) ground state, while the 8c site reveals a Gamma(8) ground state. This is in contrast to the situation found in the analogous compound Ce3Pd20Ge6, where the Gamma(8) ground state is realized for both Ce sites. In addition, these results reveal an interaction between the 8c and 4a sites previously believed to be absent. The ground state was probed with uniaxial polarization analysis across the region in which field-induced quantum criticality has previously been determined. In zero applied magnetic field no long-range magnetic order could be determined. However, further evidence of field-induced quantum criticality is presented with the observation of diffuse scattering consistent with quantum fluctuations due to nearest-neighbor spin correlations between the two Ce sites.

引用

页数：8

共 32 条

[21] RAISING OF ANGULAR MOMENTUM DEGENERACY OF F-ELECTRON TERMS BY CUBIC CRYSTAL FIELDS [J].

LEA, KR ;

LEASK, MJM ;

WOLF, WP .

JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS, 1962, 23 (OCT) :1381-&

[22]

Murani A. P., 1987, Theoretical and Experimental Aspects of Valence Fluctuations. Proceedings of the Fifth International Conference on Valence Fluctuations, P287

[23] First neutron measurements on Ce3Pd20Si6 [J].

Paschen, S. ;

Laurnann, S. ;

Prokofieva, A. ;

Strydorn, A. M. ;

Deen, P. P. ;

Stewart, J. R. ;

Neumaier, K. ;

Goukassov, A. ;

Mignot, J. -M. .

PHYSICA B-CONDENSED MATTER, 2008, 403 (5-9) :1306-1308

[24] Quantum critical behaviour in Ce3Pd20Si6? [J].

Paschen, S. ;

Mueller, M. ;

Custers, J. ;

Kriegisch, M. ;

Prokofiev, A. ;

Hilscher, G. ;

Steiner, W. ;

Pikul, A. ;

Steglich, F. ;

Strydom, A. M. .

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 2007, 316 (01) :90-92

[25]

Paschen S., 2006, THERMOELECTRICS HDB

[26]

RAINFORD BD, 1982, J PHYS-PARIS, V43, pC7

[27]

Squires G. L., 1978, Introduction to The Theory of Thermal Neutron Scattering

[28] MATRIX ELEMENTS AND OPERATOR EQUIVALENTS CONNECTED WITH THE MAGNETIC PROPERTIES OF RARE EARTH IONS [J].

STEVENS, KWH .

PROCEEDINGS OF THE PHYSICAL SOCIETY OF LONDON SECTION A, 1952, 65 (387) :209-215

[29] Disordered materials studied using neutron polarization analysis on the multi-detector spectrometer, D7 [J].

Stewart, J. R. ;

Deen, P. P. ;

Andersen, K. H. ;

Schober, H. ;

Barthelemy, J. -F. ;

Hillier, J. M. ;

Murani, A. P. ;

Hayes, T. ;

Lindenau, B. .

JOURNAL OF APPLIED CRYSTALLOGRAPHY, 2009, 42 :69-84

[30] Possible field-induced quantum criticality in Ce3Pd20Si6 [J].

Strydom, A. M. ;

Pikul, A. ;

Steglich, F. ;

Paschen, S. .

YAMADA CONFERENCE LX ON RESEARCH IN HIGH MAGNETIC FIELDS, 2006, 51 :239-+

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