1-Methyl-1,4-cyclohexadiene as a Traceless Reducing Agent for the Synthesis of Catechols and Hydroquinones

被引:18
作者
Baschieri, Andrea [1 ]
Amorati, Riccardo [1 ]
Valgimigli, Luca [1 ]
Sambri, Letizia [2 ]
机构
[1] Univ Bologna, Dipartimento Chim G Ciamician, Via S Giacomo 11, I-40126 Bologna, Italy
[2] Univ Bologna, Dipartimento Chim Ind T Montanari, Viale Risorgimento 4, I-40136 Bologna, Italy
关键词
UNCATALYZED TRANSFER HYDROGENATION; ANTIOXIDANT ACTIVITY; DONATING ABILITY; QUINONES; RADICALS; CATALYST; PHENOLS; REARRANGEMENT; BIOSYNTHESIS; DERIVATIVES;
D O I
10.1021/acs.joc.9b01898
中图分类号
O62 [有机化学];
学科分类号
070303 ; 081704 ;
摘要
Pro-aromatic and volatile 1-methyl-1,4-cyclohexadiene (MeCHD) was used for the first time as a valid H-atom source in an innovative method to reduce ortho or para quinones to obtain the corresponding catechols and hydroquinones in good to excellent yields. Notably, the excess of MeCHD and the toluene formed as the oxidation product can be easily removed by evaporation. In some cases, trifluoroacetic acid as a catalyst was added to obtain the desired products. The reaction proceeds in air and under mild conditions, without metal catalysts and sulfur derivatives, resulting in an excellent and competitive method to reduce quinones. The mechanism is attributed to a radical reaction triggered by a hydrogen atom transfer from MeCHD to quinones, or, in the presence of trifluoroacetic acid, to a hydride transfer process.
引用
收藏
页码:13655 / 13664
页数:10
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