Infrared Induced Reactivity on the Surface of Isolated Size-Selected Clusters: Dissociation of N2O on Rhodium Clusters

被引：71

作者：

Hamilton, Suzanne M. ^{[1
]}

Hopkins, W. Scott ^{[1
]}

Harding, Dan J. ^{[2
,3
,4
]}

Walsh, Tiffany R. ^{[2
,3
]}

Gruene, Philipp ^{[4
]}

Haertelt, Marko ^{[4
]}

Fielicke, Andre ^{[4
]}

Meijer, Gerard ^{[4
]}

Mackenzie, Stuart R. ^{[1
]}

机构：

[1] Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, Oxford OX1 3QZ, England

[2] Univ Warwick, Dept Chem, Coventry CV4 7AL, W Midlands, England

[3] Univ Warwick, Ctr Comp Sci, Coventry CV4 7AL, W Midlands, England

[4] Max Planck Gesell, Fritz Haber Inst, D-14195 Berlin, Germany

来源：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2010年 / 132卷 / 05期

基金：

英国工程与自然科学研究理事会;

关键词：

VIBRATIONAL SPECTROSCOPY; NITROUS-OXIDE; GAS-PHASE; ADSORPTION; CATIONS; CO; DECOMPOSITION; DESORPTION; COMPLEXES; IONS;

D O I：

10.1021/ja907496c

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Multiple photon infrared excitation of size-selected Rh6N2O+ clusters drives surface chemistry resulting in partially oxidized Clusters.

引用

页码：1448 / +

页数：4

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