Extreme optical chirality of plasmonic nanohole arrays due to chiral Fano resonance

被引:60
作者
Kondratov, A. V. [1 ]
Gorkunov, M. V. [1 ,2 ]
Darinskii, A. N. [1 ]
Gainutdinov, R. V. [1 ]
Rogov, O. Y. [1 ]
Ezhov, A. A. [1 ,3 ]
Artemov, V. V. [1 ]
机构
[1] Russian Acad Sci, Fed Sci Res Ctr Crystallog & Photon, AV Shubnikov Crystallog Inst, Moscow 119333, Russia
[2] Natl Res Nucl Univ MEPhI, Moscow Engn Phys Inst, Moscow 115409, Russia
[3] Moscow MV Lomonosov State Univ, Fac Phys, Moscow 119991, Russia
基金
俄罗斯科学基金会;
关键词
METAL NANOPARTICLES; CIRCULAR POLARIZERS; METAMATERIALS; SCALE;
D O I
10.1103/PhysRevB.93.195418
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We study the physical origin of extreme optical chirality of subwavelength arrays of chiral holes in metal. We reconstruct the nanoscale relief of the hole arrays by the atomic-force microscopy and post-process the data to acquire an average unit-cell shape clear of noise and defects. For this shape, we perform the electromagnetic finite difference time domain simulations that reproduce all important features observed by the light-transmission experiments, including the notably strong circular dichroism and optical activity covering the whole range of possible values. To interpret the simulation results, we develop a chiral coupled-mode model which yields analytical expressions that fit accurately the numerical data in a broad wavelength range. Our conclusions undoubtedly link the extreme optical chirality to the plasmon resonances of chiral holes and the associated chiral Fano-type transmission resonance.
引用
收藏
页数:10
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