Exciton dynamics in WSe2 bilayers

被引:52
作者
Wang, G. [1 ]
Marie, X. [1 ]
Bouet, L. [1 ]
Vidal, M. [1 ]
Balocchi, A. [1 ]
Amand, T. [1 ]
Lagarde, D. [1 ]
Urbaszek, B. [1 ]
机构
[1] Univ Toulouse, INSA CNRS UPS, LPCNO, F-31077 Toulouse, France
关键词
FEW-LAYER MOS2; VALLEY POLARIZATION; MONO LAYER; SPIN; COHERENCE; WS2;
D O I
10.1063/1.4900945
中图分类号
O59 [应用物理学];
学科分类号
摘要
We investigate exciton dynamics in WSe2 bilayers in time-resolved photoluminescence (PL) spectroscopy. Fast PL emission times are recorded for both the direct exciton with tau(D) less than or similar to 3 ps and the indirect optical transition with tau(I) approximate to 25 ps. For temperatures between 4 to 150K tau(I) remains constant. Following polarized laser excitation, we observe for the direct exciton transition at the K point of the Brillouin zone efficient optical orientation and alignment during the short emission time tau(D). The evolution of the direct exciton polarization and intensity as a function of excitation laser energy is monitored in PL excitation experiments. (C) 2014 AIP Publishing LLC.
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页数:4
相关论文
共 44 条
[1]   Valley-selective circular dichroism of monolayer molybdenum disulphide [J].
Cao, Ting ;
Wang, Gang ;
Han, Wenpeng ;
Ye, Huiqi ;
Zhu, Chuanrui ;
Shi, Junren ;
Niu, Qian ;
Tan, Pingheng ;
Wang, Enge ;
Liu, Baoli ;
Feng, Ji .
NATURE COMMUNICATIONS, 2012, 3
[2]   Quasiparticle band structure calculation of monolayer, bilayer, and bulk MoS2 [J].
Cheiwchanchamnangij, Tawinan ;
Lambrecht, Walter R. L. .
PHYSICAL REVIEW B, 2012, 85 (20)
[3]   Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS2 [J].
Chernikov, Alexey ;
Berkelbach, Timothy C. ;
Hill, Heather M. ;
Rigosi, Albert ;
Li, Yilei ;
Aslan, Ozgur Burak ;
Reichman, David R. ;
Hybertsen, Mark S. ;
Heinz, Tony F. .
PHYSICAL REVIEW LETTERS, 2014, 113 (07)
[4]   Electronic structure of two-dimensional transition metal dichalcogenide bilayers from ab initio theory [J].
Debbichi, L. ;
Eriksson, O. ;
Lebegue, S. .
PHYSICAL REVIEW B, 2014, 89 (20)
[5]   High-temperature superfluidity with indirect excitons in van der Waals heterostructures [J].
Fogler, M. M. ;
Butov, L. V. ;
Novoselov, K. S. .
NATURE COMMUNICATIONS, 2014, 5
[6]   Van der Waals heterostructures [J].
Geim, A. K. ;
Grigorieva, I. V. .
NATURE, 2013, 499 (7459) :419-425
[7]   Exciton fine structure and spin decoherence in monolayers of transition metal dichalcogenides [J].
Glazov, M. M. ;
Amand, T. ;
Marie, X. ;
Lagarde, D. ;
Bouet, L. ;
Urbaszek, B. .
PHYSICAL REVIEW B, 2014, 89 (20)
[8]  
HARLE V, 1994, SIXTH INTERNATIONAL CONFERENCE ON INDIUM PHOSPHIDE AND RELATED MATERIALS: CONFERENCE PROCEEDINGS, P6, DOI 10.1109/ICIPRM.1994.328146
[9]   Tightly Bound Excitons in Monolayer WSe2 [J].
He, Keliang ;
Kumar, Nardeep ;
Zhao, Liang ;
Wang, Zefang ;
Mak, Kin Fai ;
Zhao, Hui ;
Shan, Jie .
PHYSICAL REVIEW LETTERS, 2014, 113 (02)
[10]   Direct Measurement of the Thickness-Dependent Electronic Band Structure of MoS2 Using Angle-Resolved Photoemission Spectroscopy [J].
Jin, Wencan ;
Yeh, Po-Chun ;
Zaki, Nader ;
Zhang, Datong ;
Sadowski, Jerzy T. ;
Al-Mahboob, Abdullah ;
van der Zande, Arend M. ;
Chenet, Daniel A. ;
Dadap, Jerry I. ;
Herman, Irving P. ;
Sutter, Peter ;
Hone, James ;
Osgood, Richard M., Jr. .
PHYSICAL REVIEW LETTERS, 2013, 111 (10)