Exploring the link between molecular cloud ices and chondritic organic matter in laboratory

被引:18
作者
Danger, G. [1 ,2 ,3 ]
Vinogradoff, V. [1 ,2 ]
Matzka, M. [4 ,5 ]
Viennet, J-C. [6 ]
Remusat, L. [6 ]
Bernard, S. [6 ]
Ruf, A. [1 ]
d'Hendecourt, L. Le Sergeant [1 ,2 ]
Schmitt-Kopplin, P. [4 ,5 ]
机构
[1] Aix Marseille Univ, CNRS, UMR 7345, Lab Phys Interact Ion & Mol, Marseille, France
[2] Aix Marseille Univ, CNRS, UMR 7326, Lab Astrophys Marseille,CNES, Marseille, France
[3] Inst Univ France IUF, Paris, France
[4] Helmholtz Zentrum Munchen, Analyt BioGeoChem, Neuherberg, Germany
[5] Tech Univ Munich, Chair Analyt Food Chem, Freising Weihenstephan, Germany
[6] Sorbonne Univ, UMR CNRS 7590, Inst Mineral Phys Mat & Cosmochim, Museum Natl Hist Nat, Paris, France
基金
欧洲研究理事会;
关键词
AQUEOUS ALTERATION; HYDROTHERMAL ALTERATION; INTERSTELLAR; ANALOGS; ORIGIN; METEORITES; CHEMISTRY; EVOLUTION; MURCHISON; CM;
D O I
10.1038/s41467-021-23895-2
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Carbonaceous meteorites are fragments of asteroids rich in organic material. In the forming solar nebula, parent bodies may have accreted organic materials resulting from the evolution of icy grains observed in dense molecular clouds. The major issues of this scenario are the secondary processes having occurred on asteroids, which may have modified the accreted matter. Here, we explore the evolution of organic analogs of protostellar/protoplanetary disk material once accreted and submitted to aqueous alteration at 150 degrees C. The evolution of molecular compounds during up to 100 days is monitored by high resolution mass spectrometry. We report significant evolution of the molecular families, with the decreases of H/C and N/C ratios. We find that the post-aqueous products share compositional similarities with the soluble organic matter of the Murchison meteorite. These results give a comprehensive scenario of the possible link between carbonaceous meteorites and ices of dense molecular clouds. Several scenarios exist to explain the origins of the organic matter found in carbonaceous chondrites. Here, the authors show laboratory experiments confirming that a significant portion of the soluble organic matter can originate from organic ices inherited from the dense molecular cloud.
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页数:9
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