Carbon-nitrogen-metal material as a high performing oxygen evolution catalyst

被引：0

作者：

Fruehwald, Holly M. ^{[1
]}

Zenkina, Olena V. ^{[1
]}

Easton, E. Bradley ^{[1
]}

机构：

[1] Univ Ontario, Ontario Tech Univ, Inst Technol, Fac Sci, 2000 Simcoe St North, Oshawa, ON L1G 0C5, Canada

来源：

CATALYSIS SCIENCE & TECHNOLOGY | 2022年 / 12卷 / 10期

基金：

加拿大自然科学与工程研究理事会;

关键词：

HYDROGEN EVOLUTION; GRAPHENE OXIDE; NANOPARTICLES; HYDROXIDES; REDUCTION;

D O I：

10.1039/d2cy00473a

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Novel oxygen evolution catalysts were prepared through diazonium coupling chemistry to covalently modify Vulcan carbon via terpyridine (tpy) motifs followed by coordination of non-precious transition metals (Ni, Co) to the tpy-ligand on the surface support. This resulted in highly active catalysts that demonstrate low overpotentials for the V-tpy-Ni catalyst of 313 mV at 10 mA cm(-2), and stable long-term performance over 26 hours of continual testing.

引用

页码：3102 / 3105

页数：4

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