Synthesis of Hierarchical Graphdiyne-Based Architecture for Efficient Solar Steam Generation

被引:221
作者
Gao, Xin [1 ]
Ren, Huaying [1 ,2 ]
Zhou, Jingyuan [1 ,2 ]
Du, Ran [1 ]
Yin, Chen [1 ,2 ]
Liu, Rong [1 ,2 ]
Peng, Hailin [1 ]
Tong, Lianming [1 ]
Liu, Zhongfan [1 ]
Zhang, Jin [1 ]
机构
[1] Peking Univ, Ctr Nanochem, Beijing Sci & Engn Ctr Nanocarbons, BNLMS,Coll Chem & Mol Engn, Beijing 100871, Peoples R China
[2] Peking Univ, Acad Adv Interdisciplinary Studies, Beijing 100871, Peoples R China
基金
中国国家自然科学基金;
关键词
THEORETICAL PREDICTIONS; HEAT LOCALIZATION; DESALINATION; EVAPORATION; GRAPHENE; NANOPARTICLES; SUBSTRATE; GRAPHYNE; STORAGE;
D O I
10.1021/acs.chemmater.7b01838
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A study has been conducted to develop a new structure based on three-dimensional (3D) copper foam supported one-dimensional (1D) CuO nanowires anchoring with vertical twodimensional (2D) GDY nanosheets. In this architecture, the copper foam provides the self-supporting sketelon, CuO nanowires are responsible for most solar absorption, and GDY nanosheets could simultaneously trap the light via structual factors and enhance the light absorption through its intrinsic narrow band gap. As a result, a photothermal conversion efficiency of up to 91% has been achieved, making this GDY-based structure promising not only for efficient solar steam generation but also in diverse fields such as water desalination and environmental remediation.
引用
收藏
页码:5777 / 5781
页数:5
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